光电子谱技术是研究原子、分子、固体和表面电子
结构的一种非常有效的手段。本书全面
系统地介绍了
光电子谱技术的
原理和应用,并简明讨论了逆光发射、自旋极化光发射和
光电子衍射等现象。本书是一本非常实用的光电子谱技术的专著,内容几乎覆盖了光电子研究的所有领域。其特点是紧密联系实验,并利用理论详细解释实验结果,达到理论和应用的有机结合。书中还收集了大量的实际
材料的光电子谱分析,同时给出了大量的实验数据,以便于读者的查阅。总之,该书既是一本很有价值的参考书,又可作为初学者的入门教材。
COF_a% m3cO{
1I 作者在该领域做出了杰出的贡献。在第3版中,作者介绍了大量最新研究成果,并对光电子谱技术很多方面给出了有深刻见解的讨论。
`H_.<``> [M7& 读者对象:适用于凝聚态
物理学、材料物理学和光电子学等专业的高年级本科生、研究生和相关专业的科研人员。
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3kl<~O|Fs Z`?Z1SBt 目录
80p? qe 1. Introduction and Basic Principles
rW~hFSrV[o 1.1 Historical Development
$[p<}o/6v] 1.2 The Electron Mean Free Path
9q##) 1.3 Photoelectron Spectroscopy and Inverse Photoelectron Spectroscopy
'q#$^='o 1.4 Experimental Aspects
&m>yY{be 1.5 Very High Resolution
Eagl7'x 1.6 The Theory of Photoemission
Ux<2!vh 1.6.1 Core-Level Photoemission
_o
2pyV& 1.6.2 Valence-State Photoemission
8f^QO: 1.6.3 Three-Step and One-Step Considerations
PWwz<AI+ 1.7 Deviations from the Simple Theory of Photoemission
"1<>c/h References
;Y&<psQeb 44uM:; 2. Core Levels and Final States
`30og]F0YJ 2.1 Core-Level Binding Energies in Atoms and Molecules
rj.]M6# 2.1.1 The Equivalent-Core Approximation
f`8]4ms" 2.1.2 Chemical Shifts
[@l:C\2 2.2 Core-Level Binding Energies in Solids
+}XFkH~ 2.2.1 The Born-Haber Cycle in Insulators
1@ e22\ 2.2.2 Theory of Binding Energies
sd@JQ%O 2.2.3 Determination of Binding Energies and Chemical Shifts from Thermodynamic Data
k63]Qf=5?N 2.3 Core Polarization
Q:
H`TSR] 2.4 Final-State Multiplets in Rare-Earth Valence Bands
y?ps+ce93 2.5 Vibrational Side Bands
F~NmLm 2.6 Core Levels of Adsorbed Molecules
d!V;\w 2.7 Quantitative Chemical Analysis from Core-Level Intensities
'Xl_,;W] References
S(K}.C1x Px!M^
T!Pi 3. Charge-Excitation Final States: Satellites
Rmq8lU 3.1 Copper Dihalides; 3d Transition Metal Compounds
v4?qI >/ 3.1.1 Characterization of a Satellite
q'07 3.1.2 Analysis of Charge-Transfer Satellites
kIm)Um 3.1.3 Non-local Screening
6' 9ITA 3.2 The 6-eV Satellite in Nickel
Mw0Kg9M 3.2.1 Resonance Photoemission
duCso M/ 3.2.2 Satellites in Other Metals
q8 j
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X=:|v<E
3.4 Photoemission Signals and Narrow Bands in Metals
JGJXV3AT References
W[5a'}OV _I("k:E7 4. Continuous Satellites and Plasmon Satellites: XPS Photoemission in Nearly Free Electron Systems
6#,VnS)`q 4.1 Theory
n9Mi?#xIp 4.1.1 General
=~)J:x\F 4.1.2 Core-Line Shape
,rvw E 4.1.3 Intrinsic Plasmons
Dr;-2$Kt/& 4.1.4 Fxtrinsic FAectron Scattering: Plasmons and Background
E>/kNl 4.1.5 The Total Photoelectron Spectrum
b(hnou S 4.2 Experimental Results
H5L~[\
5t 4.2.1 The Core Line Without Plasmons
QKj-"y[ 4.2.2 Core-Level Spectra Including Plasmoas
IZ<d~ [y 4.2.3 Valence-Band Spectra of the Simple Metals
Ig9gGI, 4.2.4 Simple Metals: A General Comment
//SH=>w2 4.3 The Background Correction
Ueq*R(9> References
px@:t} $ekB+
t:cj 5. Valence Orbitals in Simple Molecules and Insulating Solids
ZT
UaF4k j 5.1 UPS Spectra of Monatomic Gases
PT9,R^2T! 5.2 Photoelectron Spectra of Diatomic Molecules
uR|?5DK 5.3 Binding Energy of the H2 Molecule
r<Il;?S6 5.4 Hydrides Isoelectronic with Noble Gases
mN>7vJ Neon (Ne)
th@a./h" Hydrogen Fluoride (HF)
<<43'N+ Water (H2O)
~0mO<0~ Ammonia (NH3)
SF$]{
X Methane (CH4)
qIbp0`m 5.5 Spectra of the Alkali HMides
*Q?ZJS~ 5.6 Transition Metal Dihalides
h0YIPB 5.7 Hydrocarbons
n:hHm, 5.7.1 Guidelines for the Interpretation of Spectra from Free Molecules
8PWx>}XPt 5.7.2 Linear Polymers
6g/ <FM 5.8 Insulating Solids with Valence d Electrons
VDCG
5QP6( 5.8.1 The NiO Problem
%SV5PO@ 5.8.2 Mort Insulation
&<!DNXQ 5.8.3 The Metal-Insulator Transition;the Ratio of the Correlation Energy and the Bandwidth;Doping
o80"ZU|= 5.8.4Band Structures of Transition Metal Compounds
'A0.(a5 5.9 High—Temperature Superconductors
`rt 5.9.1valence-Band Electronic Structure;Polycrystalline Samples
()< E?D= 5.9.2 Dispersion Relations in High Temperature Superconductors;Single Crystals
kB|jN~ 5.9.3 The Superconducting Gap
E7A psi4] 5.9.4 Symmetry of the Order Parameter in the High-Temperature SuDerconductors
C2WWS(zn 5.9.5 Core—Level Shifts
U@W3x@ 5.10 The Fermi Liquid and the Luttinger Liquid
?(9/V7HQ.5 5.11 Adsorbed Molecules
\a:#e%]qz9 5.11.1 Outline
Y\7>>? 5.11.2 CO on Metal Surfaces
e rz9CX References
H4s^&-- TU6e,G|t 6.Photoemission of Valence Electrons froill Metallic Solids in the OHe-Electron Approximation
X^!n'$^u 6.1 Theory of Photoemission:A Summary of the Three-Step Model
J%G
EIe| 6.2 Discussion of the Photocurrent
Vy]y73~ 6.2.1 Kinematics of Internal Photoemission in a Polycrystalline Sample
)ZxDfRjL 6.2.2 Primary and Secondary Cones in the Photoemission from a Real Solid
]*I:N 6.2.3 Angle-Integrated and Angle-Resolved Data Collection
VO_! + 6.3 Photoemission from the Semi—infinite Crystal:The Inverse LEED Formalism
=x9SvIm/tH 6.3.1 Band Structure Regime
e):jQite
6.3.2 XPS Regime
U 6(( 6.3.3 Surface Emission
VR86ok 6.3.4 One-Step Calculations
M2K{{pGJ[& 6.4 Thermal Effects
yN9k-IPI 6.5 Dipole Selection Rules for Direct Optical Transitions
;x 9_ References
hf6=`M}>i \#LkzN8 7.Band Structtire and Angular-Resolved Photoelectron Spectra
~U] "dbQ 7.1 Free-Electron Final—State Model
1 &24:& 7.2 Methods Employing Calculated Band Structures
>FO4] 7.3 Methods for the Absolute Determination of the Crystal Momentum
_lWC)bv` 7.3.1 Triangulation or Energy Coincidence Method
d~i WV6Va 7.3.2 Bragg Plane Method: Variation of External Emission Angle at Fixed Photon Frequency (Disappearance/Appearance Angle Method
,EkzBVgo 7.3.3 Bragg Plane Method: Variation of Photon Energy at Fixed Emission Angle (Symmetry Method)
~vqVASUc, 7.3.4 The Surface Emission Method and Electron Damping
zV)(i<Q 7.3.5 The Very-Low-Energy Electron Diffraction Method
3AKT>Wy = 7.3.6 The Fermi Surface Method
~7!=<MW 7.3.7 Intensities and Their Use in Band-Structure Determinations
q|An 7.3.8 Summary
&h(>jY7b; 7.4 Experimental Band Structures
XRZj+muTZ 7.4.1 One- and Two-Dimensional Systems
"gm[q."n< 7.4.2 Three-Dimensional Solids: Metals and Semiconductors
_|f1q 7..4.3UPS Band Structures and XPS Density of States
lSMv9:N 7.5 A Comment
?hqHTH:PU References
D{-h2=V G`n|fuv 8.Surface States, Surface Effects
#[|~m;K(w 8.1 Theoretical Considerations
nkI+"$Rz0 8.2 Experimental Results on Surface States
p~Tp=d)/ 8.3 Quantum-Well States
kF%EJuu 8.4 Surface Core-Level Shifts
Gv
'; References
6`KR UL9]LEGG
9.Inverse Photoelectron Spectroscopy
Rm@#GP`
9.1 Surface States
[v@3|@ 9.2 Bulk Band Structures
~q5aMy d< 9.3 Adsorbed Molecules
1D*oXE9Ig References
r7Vt,{4/ &cZQ,o 10. Spin-Polarized Photoelectron Spectroscopy
C%2BDj 10.1 General Description
kJQH{n+)R 10.2 Examples of Spin-Polarized Photoelectron Spectroscopy
r]h>Bb 10.3 Magnetic Dichroism
g=Gd| References
a
~s:f5S> D4@).% 11. Photoelectron Diffraction
o#"U8N%r 11.1 Examples
#7 )&` 11.2 Substrate Photoelectron Diffraction
myq@X(K 11.3 Adsorbate Photoelectron Diffraction
#'DrgZ)W 11.4 Fermi Surface Scans
@nC][gNv References
Cz1Q@<) :B^YK]. Appendix
mu#IF'|b A.1 Table of Binding Energies
1 X8P v*, A.2 Surface and Bulk Brillouin Zones of the Three Low-Index Faces of a Face—Centered Cubic(fcc)Crystal Face
lu_kir~ A.3 Compilation of Work Functions
OC?a[^hB^) References
tTjadnX Index