光电子谱技术是研究原子、分子、固体和表面电子
结构的一种非常有效的手段。本书全面
系统地介绍了
光电子谱技术的
原理和应用,并简明讨论了逆光发射、自旋极化光发射和
光电子衍射等现象。本书是一本非常实用的光电子谱技术的专著,内容几乎覆盖了光电子研究的所有领域。其特点是紧密联系实验,并利用理论详细解释实验结果,达到理论和应用的有机结合。书中还收集了大量的实际
材料的光电子谱分析,同时给出了大量的实验数据,以便于读者的查阅。总之,该书既是一本很有价值的参考书,又可作为初学者的入门教材。
Z;'5A2 bukdyo;l 作者在该领域做出了杰出的贡献。在第3版中,作者介绍了大量最新研究成果,并对光电子谱技术很多方面给出了有深刻见解的讨论。
uO^,N**R# lVptA3F 读者对象:适用于凝聚态
物理学、材料物理学和光电子学等专业的高年级本科生、研究生和相关专业的科研人员。
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q1Sr#h|
+,q#'wSQG 9z'(4U 目录
r"4&.&6 1. Introduction and Basic Principles
NG+%H1!$_ 1.1 Historical Development
D~Rv"Hh 1.2 The Electron Mean Free Path
FlyRcj 1.3 Photoelectron Spectroscopy and Inverse Photoelectron Spectroscopy
s=8$h:^9> 1.4 Experimental Aspects
PP{s&( 1.5 Very High Resolution
q.:j
yj6 1.6 The Theory of Photoemission
nvInq2T1 1.6.1 Core-Level Photoemission
]K-B#D{P 1.6.2 Valence-State Photoemission
#&sw%CD 1.6.3 Three-Step and One-Step Considerations
P[K42mm 1.7 Deviations from the Simple Theory of Photoemission
?910ki_ References
oK@_
UA3!28Y&E3 2. Core Levels and Final States
Q=u [j|0mc 2.1 Core-Level Binding Energies in Atoms and Molecules
$aC%&&+wG 2.1.1 The Equivalent-Core Approximation
{>h,@ 2.1.2 Chemical Shifts
]|8*l]oc 2.2 Core-Level Binding Energies in Solids
FT;I|+H*P 2.2.1 The Born-Haber Cycle in Insulators
!*!i&0QC~R 2.2.2 Theory of Binding Energies
*|B5,Ey 2.2.3 Determination of Binding Energies and Chemical Shifts from Thermodynamic Data
j
V'~> 2.3 Core Polarization
D6fGr$(N% 2.4 Final-State Multiplets in Rare-Earth Valence Bands
dTVh{~/ 2.5 Vibrational Side Bands
gg?O0W{ 2.6 Core Levels of Adsorbed Molecules
u`gY/]y! 2.7 Quantitative Chemical Analysis from Core-Level Intensities
z{(c-7* References
WqRaD=R->;
3J}/<&wv 3. Charge-Excitation Final States: Satellites
OrRU$5Lo 3.1 Copper Dihalides; 3d Transition Metal Compounds
@$7l 3.1.1 Characterization of a Satellite
92D :!C 3.1.2 Analysis of Charge-Transfer Satellites
c:u2a/Q? 3.1.3 Non-local Screening
T]lVwj 3.2 The 6-eV Satellite in Nickel
z)fg>?AGr 3.2.1 Resonance Photoemission
8,&pX ga 3.2.2 Satellites in Other Metals
{1}p+dEK 3.3 The Gunnarsson-Sch6nhammer Theory
UNCI"Mjb 3.4 Photoemission Signals and Narrow Bands in Metals
f-5}`)`.+ References
AiUK#I t-Zk)*d/0 4. Continuous Satellites and Plasmon Satellites: XPS Photoemission in Nearly Free Electron Systems
ia*Bcx_RW+ 4.1 Theory
K*aGz8N 4.1.1 General
nC@UK{tVa 4.1.2 Core-Line Shape
' p!\[*e 4.1.3 Intrinsic Plasmons
`{+aJ0<S 4.1.4 Fxtrinsic FAectron Scattering: Plasmons and Background
fctVJ{? 4.1.5 The Total Photoelectron Spectrum
pIgjo>K 4.2 Experimental Results
PS/00F/Ak 4.2.1 The Core Line Without Plasmons
PbIir= 4.2.2 Core-Level Spectra Including Plasmoas
+8 }p-<a 4.2.3 Valence-Band Spectra of the Simple Metals
^~DClZ 4.2.4 Simple Metals: A General Comment
*3h!&.zm 4.3 The Background Correction
s}Q*zy References
]-8yZWal r!)jxIL\ 5. Valence Orbitals in Simple Molecules and Insulating Solids
q/dja 5.1 UPS Spectra of Monatomic Gases
G0Wv=tX| 5.2 Photoelectron Spectra of Diatomic Molecules
KFf6um 5.3 Binding Energy of the H2 Molecule
A08{]E#v> 5.4 Hydrides Isoelectronic with Noble Gases
q/3 )yG6s Neon (Ne)
8]A`WDO3 Hydrogen Fluoride (HF)
Pi'[d7o Water (H2O)
D`@*udn= Ammonia (NH3)
xf4`+[ Methane (CH4)
o0FVVS l 5.5 Spectra of the Alkali HMides
4L/8Hj#g 5.6 Transition Metal Dihalides
Na>?1F"KHk 5.7 Hydrocarbons
5tcJTz 5.7.1 Guidelines for the Interpretation of Spectra from Free Molecules
i1-wzI
5.7.2 Linear Polymers
C^9bur/ 5.8 Insulating Solids with Valence d Electrons
4qg]
oiT 5.8.1 The NiO Problem
zf?U q 5.8.2 Mort Insulation
^<v]x;
3 5.8.3 The Metal-Insulator Transition;the Ratio of the Correlation Energy and the Bandwidth;Doping
L<O"36R 5.8.4Band Structures of Transition Metal Compounds
(db4.G+0 5.9 High—Temperature Superconductors
MzCZj 5.9.1valence-Band Electronic Structure;Polycrystalline Samples
xYD.j~ 5.9.2 Dispersion Relations in High Temperature Superconductors;Single Crystals
4qmaL+Q 5.9.3 The Superconducting Gap
O_[]+5.TX 5.9.4 Symmetry of the Order Parameter in the High-Temperature SuDerconductors
=(]||1. 5.9.5 Core—Level Shifts
|emZZj 5.10 The Fermi Liquid and the Luttinger Liquid
ZfSAXr "( 5.11 Adsorbed Molecules
t.6gyrV7>< 5.11.1 Outline
@>Ul0&Mf? 5.11.2 CO on Metal Surfaces
tjt#2i8/ References
8L,i}hIo. Qhsk09K_=4 6.Photoemission of Valence Electrons froill Metallic Solids in the OHe-Electron Approximation
BZs?tbf 6.1 Theory of Photoemission:A Summary of the Three-Step Model
.+2@(r 6.2 Discussion of the Photocurrent
#NR9\ 6.2.1 Kinematics of Internal Photoemission in a Polycrystalline Sample
`ILO]+`5 6.2.2 Primary and Secondary Cones in the Photoemission from a Real Solid
\
0aa0= 6.2.3 Angle-Integrated and Angle-Resolved Data Collection
`'}c-
Q 6.3 Photoemission from the Semi—infinite Crystal:The Inverse LEED Formalism
|c3Yh,Sv 6.3.1 Band Structure Regime
[y1
x`WOk9 6.3.2 XPS Regime
vGI?X#w3 6.3.3 Surface Emission
UWW_[dJr 6.3.4 One-Step Calculations
YRs32vVz 6.4 Thermal Effects
DgRA\[c 6.5 Dipole Selection Rules for Direct Optical Transitions
'qnnZE References
n;0x\Q|S ;sfk@ec 7.Band Structtire and Angular-Resolved Photoelectron Spectra
h;Se.{ 7.1 Free-Electron Final—State Model
["
nDw<U 7.2 Methods Employing Calculated Band Structures
4Q5c' 7.3 Methods for the Absolute Determination of the Crystal Momentum
BZ-)XF'4 7.3.1 Triangulation or Energy Coincidence Method
)\|Bghui 7.3.2 Bragg Plane Method: Variation of External Emission Angle at Fixed Photon Frequency (Disappearance/Appearance Angle Method
[SA$d`B/ 7.3.3 Bragg Plane Method: Variation of Photon Energy at Fixed Emission Angle (Symmetry Method)
Ialbz\;F2% 7.3.4 The Surface Emission Method and Electron Damping
Gw0MDV&[ 7.3.5 The Very-Low-Energy Electron Diffraction Method
;'xd8Jf 7.3.6 The Fermi Surface Method
BHEZ<K[U
7.3.7 Intensities and Their Use in Band-Structure Determinations
n
2m!a0; 7.3.8 Summary
`Wy8g?d;bn 7.4 Experimental Band Structures
p@bcf5' 7.4.1 One- and Two-Dimensional Systems
{fAj*,pzl 7.4.2 Three-Dimensional Solids: Metals and Semiconductors
.~yz1^ c 7..4.3UPS Band Structures and XPS Density of States
&a];"2 7.5 A Comment
@gHWU>k,A References
v|K<3@J s^Wh!:>r/ 8.Surface States, Surface Effects
>Pw
ZHY 8.1 Theoretical Considerations
#Hy fjj 8.2 Experimental Results on Surface States
yHt
`kb2 8.3 Quantum-Well States
ECF \/12 8.4 Surface Core-Level Shifts
}ikJa References
SFRQpQ06 Bh*7uNM 9.Inverse Photoelectron Spectroscopy
dLIZ)16& 9.1 Surface States
6pi^ rpo 9.2 Bulk Band Structures
{9yW8&m 9.3 Adsorbed Molecules
!mLD`62. References
m_n*_tX X`E3lgfqT 10. Spin-Polarized Photoelectron Spectroscopy
WG?;Z 10.1 General Description
\"^.>+ 10.2 Examples of Spin-Polarized Photoelectron Spectroscopy
T($6L7 j9 10.3 Magnetic Dichroism
L4C_qb k;: References
"8|a4Y+F U*7Yi-"/* 11. Photoelectron Diffraction
%.3]F2_Q 11.1 Examples
>:yU bo) 11.2 Substrate Photoelectron Diffraction
0zvA>4cq) 11.3 Adsorbate Photoelectron Diffraction
"Ooc;xD3< 11.4 Fermi Surface Scans
e$+/;MRq References
eX9Hwq4X44 k yI -nE Appendix
DHnu F@M A.1 Table of Binding Energies
_>"f&nbO A.2 Surface and Bulk Brillouin Zones of the Three Low-Index Faces of a Face—Centered Cubic(fcc)Crystal Face
95%,
8t A.3 Compilation of Work Functions
(iw)C)t*u References
$pOgFA1' Index