光电子谱技术是研究原子、分子、固体和表面电子
结构的一种非常有效的手段。本书全面
系统地介绍了
光电子谱技术的
原理和应用,并简明讨论了逆光发射、自旋极化光发射和
光电子衍射等现象。本书是一本非常实用的光电子谱技术的专著,内容几乎覆盖了光电子研究的所有领域。其特点是紧密联系实验,并利用理论详细解释实验结果,达到理论和应用的有机结合。书中还收集了大量的实际
材料的光电子谱分析,同时给出了大量的实验数据,以便于读者的查阅。总之,该书既是一本很有价值的参考书,又可作为初学者的入门教材。
^c^#dpn El.hu%#n*G 作者在该领域做出了杰出的贡献。在第3版中,作者介绍了大量最新研究成果,并对光电子谱技术很多方面给出了有深刻见解的讨论。
|=`~-i2W %s|}Fz-> 读者对象:适用于凝聚态
物理学、材料物理学和光电子学等专业的高年级本科生、研究生和相关专业的科研人员。
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b:lP%|7 QdL`| 目录
&PYK8}pBk3 1. Introduction and Basic Principles
W6?pswQ 1.1 Historical Development
S ?{#r 1.2 The Electron Mean Free Path
*AO,^R&e. 1.3 Photoelectron Spectroscopy and Inverse Photoelectron Spectroscopy
2R;}y7{ 1.4 Experimental Aspects
qf!p 9@4F[ 1.5 Very High Resolution
p"n$!ilbm 1.6 The Theory of Photoemission
,z;cbsV-{ 1.6.1 Core-Level Photoemission
wy0tgy(' | 1.6.2 Valence-State Photoemission
kCR_tn
4 1.6.3 Three-Step and One-Step Considerations
*=]&&< 1.7 Deviations from the Simple Theory of Photoemission
^@3sT,M,S References
'p>Ra/4 B@&4i?yJ 2. Core Levels and Final States
/67 h&j 2.1 Core-Level Binding Energies in Atoms and Molecules
(.D~0a JU 2.1.1 The Equivalent-Core Approximation
nuk*.Su 2.1.2 Chemical Shifts
,]46I.] 2.2 Core-Level Binding Energies in Solids
[x+FcXb 2.2.1 The Born-Haber Cycle in Insulators
oW ::hB 2.2.2 Theory of Binding Energies
dIN$)?aB0 2.2.3 Determination of Binding Energies and Chemical Shifts from Thermodynamic Data
d:BG#\e]v 2.3 Core Polarization
coW:DFX 2.4 Final-State Multiplets in Rare-Earth Valence Bands
B8": 2HrW$ 2.5 Vibrational Side Bands
(gP)% 2.6 Core Levels of Adsorbed Molecules
R=gb' 2.7 Quantitative Chemical Analysis from Core-Level Intensities
l`oZ)?ur References
QRHu3w 9oYgl1}d 3. Charge-Excitation Final States: Satellites
ZrPbl"`7 3.1 Copper Dihalides; 3d Transition Metal Compounds
'[AlhBX 3.1.1 Characterization of a Satellite
)c8rz[i 3.1.2 Analysis of Charge-Transfer Satellites
jrr EAp 3.1.3 Non-local Screening
h2Ld[xvCu% 3.2 The 6-eV Satellite in Nickel
>AVVEv18 3.2.1 Resonance Photoemission
&]`(v}`] 3.2.2 Satellites in Other Metals
3EJj9}#x"' 3.3 The Gunnarsson-Sch6nhammer Theory
[pbo4e,4O 3.4 Photoemission Signals and Narrow Bands in Metals
[<n2Uz7MP References
zk$FkbX b$N2z 4. Continuous Satellites and Plasmon Satellites: XPS Photoemission in Nearly Free Electron Systems
>3p\m 4.1 Theory
Bt@^+vH ~ 4.1.1 General
01wX `"I 4.1.2 Core-Line Shape
cG[l!Z 4.1.3 Intrinsic Plasmons
Of*Pw[vD 4.1.4 Fxtrinsic FAectron Scattering: Plasmons and Background
C 3^JAP 4.1.5 The Total Photoelectron Spectrum
!%CWZZ 6u 4.2 Experimental Results
Hx"ob_^'7 4.2.1 The Core Line Without Plasmons
7''??X 4.2.2 Core-Level Spectra Including Plasmoas
&XIt5<$~R 4.2.3 Valence-Band Spectra of the Simple Metals
t<#TJ>Le 4.2.4 Simple Metals: A General Comment
uaT!(Y6 4.3 The Background Correction
aOlT;h References
my(2;IJ#{ mWoAO@}Y 5. Valence Orbitals in Simple Molecules and Insulating Solids
/)YNs7gR 5.1 UPS Spectra of Monatomic Gases
2;k*@k-t 5.2 Photoelectron Spectra of Diatomic Molecules
JZ)RGSG i 5.3 Binding Energy of the H2 Molecule
vx>b^tJKC 5.4 Hydrides Isoelectronic with Noble Gases
4w*Skl=F} Neon (Ne)
a!a-b~#cx Hydrogen Fluoride (HF)
5x5@t
: Water (H2O)
,)0H3t Ammonia (NH3)
;Y00TGU Methane (CH4)
sd*p/Q|4 5.5 Spectra of the Alkali HMides
h}[-'>{ 5.6 Transition Metal Dihalides
%'bM){ 5.7 Hydrocarbons
~-ia+A6GIV 5.7.1 Guidelines for the Interpretation of Spectra from Free Molecules
<CS(c|7 5.7.2 Linear Polymers
5 h-@|t 5.8 Insulating Solids with Valence d Electrons
2M.fLQ? 5.8.1 The NiO Problem
bGN:=Y' 5.8.2 Mort Insulation
`95r0t0hh\ 5.8.3 The Metal-Insulator Transition;the Ratio of the Correlation Energy and the Bandwidth;Doping
&-;4.op 5.8.4Band Structures of Transition Metal Compounds
PRx8I
. 5.9 High—Temperature Superconductors
+9M^7/}H 5.9.1valence-Band Electronic Structure;Polycrystalline Samples
X3{G:H0\p 5.9.2 Dispersion Relations in High Temperature Superconductors;Single Crystals
caIL&G, 5.9.3 The Superconducting Gap
@@R7p 5.9.4 Symmetry of the Order Parameter in the High-Temperature SuDerconductors
sZjQ3*<-r 5.9.5 Core—Level Shifts
+[M6X}
TQ 5.10 The Fermi Liquid and the Luttinger Liquid
o*-)Tq8GHE 5.11 Adsorbed Molecules
QX!-B 5.11.1 Outline
U bXh,QEG* 5.11.2 CO on Metal Surfaces
dzARI` References
`tBgH_$M caU0\VS 6.Photoemission of Valence Electrons froill Metallic Solids in the OHe-Electron Approximation
%aHB"vi6 6.1 Theory of Photoemission:A Summary of the Three-Step Model
$:8x(&+/@ 6.2 Discussion of the Photocurrent
>tYm+coS 6.2.1 Kinematics of Internal Photoemission in a Polycrystalline Sample
/z4$gb7Y 6.2.2 Primary and Secondary Cones in the Photoemission from a Real Solid
Jb0`42 6.2.3 Angle-Integrated and Angle-Resolved Data Collection
bn#"?6Z2 6.3 Photoemission from the Semi—infinite Crystal:The Inverse LEED Formalism
? E1<!~ 6.3.1 Band Structure Regime
:y+2*lV 6.3.2 XPS Regime
Hkk/xNP 6.3.3 Surface Emission
N nRD|A 6.3.4 One-Step Calculations
iJ-23_D 6.4 Thermal Effects
]3x? 6.5 Dipole Selection Rules for Direct Optical Transitions
@'w"R/,n-@ References
w^?>e;/\ ~Y `ldL 7.Band Structtire and Angular-Resolved Photoelectron Spectra
)mg:_K 7.1 Free-Electron Final—State Model
"7
4-4 7.2 Methods Employing Calculated Band Structures
A0/"&Ag] 7.3 Methods for the Absolute Determination of the Crystal Momentum
h`]Iy 7.3.1 Triangulation or Energy Coincidence Method
xR-%L 7.3.2 Bragg Plane Method: Variation of External Emission Angle at Fixed Photon Frequency (Disappearance/Appearance Angle Method
cA2V2S) 7.3.3 Bragg Plane Method: Variation of Photon Energy at Fixed Emission Angle (Symmetry Method)
u7Y
WnD 7.3.4 The Surface Emission Method and Electron Damping
wVX[)E\J 7.3.5 The Very-Low-Energy Electron Diffraction Method
8LyD7P1\ 7.3.6 The Fermi Surface Method
]q;Emy 7.3.7 Intensities and Their Use in Band-Structure Determinations
HU1h8E$- 7.3.8 Summary
O(#)m>A 7.4 Experimental Band Structures
srr
:!5 7.4.1 One- and Two-Dimensional Systems
Pj[PIz 7.4.2 Three-Dimensional Solids: Metals and Semiconductors
l>2E (Y| 7..4.3UPS Band Structures and XPS Density of States
({
8-* 7.5 A Comment
%<)2/|lCd References
BHIRHmM<Y ^?-:'<4q$ 8.Surface States, Surface Effects
t=(!\:[D 8.1 Theoretical Considerations
&c` nR< 8.2 Experimental Results on Surface States
mf
A{3 8.3 Quantum-Well States
L(/e&J@>< 8.4 Surface Core-Level Shifts
|!1Y*|Q%s References
yd^{tQi m.JBOq= 9.Inverse Photoelectron Spectroscopy
7yG#Z)VE 9.1 Surface States
8{|8G-Mi 9.2 Bulk Band Structures
[8P:?nDDL 9.3 Adsorbed Molecules
!SC`D])l References
NC8t)
X7 -0d0t! 10. Spin-Polarized Photoelectron Spectroscopy
OPetj.C/a 10.1 General Description
aB*Bz]5;E 10.2 Examples of Spin-Polarized Photoelectron Spectroscopy
}HL]yDO 10.3 Magnetic Dichroism
m- %E-nr References
<>n0arAn 9
3U_tQ&1? 11. Photoelectron Diffraction
8|b3j^u 11.1 Examples
mH54ja2 11.2 Substrate Photoelectron Diffraction
QEm|])V 11.3 Adsorbate Photoelectron Diffraction
N@;?CKU 11.4 Fermi Surface Scans
\n" {qfn`r References
y>R=`A1b Ot$-!Y;< Appendix
Qwz}B A.1 Table of Binding Energies
Y_Eb'*PY A.2 Surface and Bulk Brillouin Zones of the Three Low-Index Faces of a Face—Centered Cubic(fcc)Crystal Face
\(~y? l A.3 Compilation of Work Functions
?RX3MUN References
\K_ET> ! Index