光电子谱技术是研究原子、分子、固体和表面电子
结构的一种非常有效的手段。本书全面
系统地介绍了
光电子谱技术的
原理和应用,并简明讨论了逆光发射、自旋极化光发射和
光电子衍射等现象。本书是一本非常实用的光电子谱技术的专著,内容几乎覆盖了光电子研究的所有领域。其特点是紧密联系实验,并利用理论详细解释实验结果,达到理论和应用的有机结合。书中还收集了大量的实际
材料的光电子谱分析,同时给出了大量的实验数据,以便于读者的查阅。总之,该书既是一本很有价值的参考书,又可作为初学者的入门教材。
!l1ycQM l+i9)Fc<i 作者在该领域做出了杰出的贡献。在第3版中,作者介绍了大量最新研究成果,并对光电子谱技术很多方面给出了有深刻见解的讨论。
<Q?X'. hKYA 5] 读者对象:适用于凝聚态
物理学、材料物理学和光电子学等专业的高年级本科生、研究生和相关专业的科研人员。
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4V0j1k&' Z'L}x6 目录
Jri"Toz0 1. Introduction and Basic Principles
Td>Lp=0rU 1.1 Historical Development
F;^GhiQVS 1.2 The Electron Mean Free Path
.ahYjn 1.3 Photoelectron Spectroscopy and Inverse Photoelectron Spectroscopy
:If1zB) 1.4 Experimental Aspects
X"qC&oZmf 1.5 Very High Resolution
%rZJ#p[e)= 1.6 The Theory of Photoemission
RtVG6'Y 1.6.1 Core-Level Photoemission
i@}/KT 1.6.2 Valence-State Photoemission
rwUKg[
1N 1.6.3 Three-Step and One-Step Considerations
?1u2P$d 1.7 Deviations from the Simple Theory of Photoemission
X}$uvB}+> References
i''[u J_^Ml)@iy 2. Core Levels and Final States
Fn~?YN 2.1 Core-Level Binding Energies in Atoms and Molecules
DpaPRA)x 2.1.1 The Equivalent-Core Approximation
G&/RJLX|w 2.1.2 Chemical Shifts
H%:~&_D 2.2 Core-Level Binding Energies in Solids
0*KU"JcXd 2.2.1 The Born-Haber Cycle in Insulators
I?mU _^no 2.2.2 Theory of Binding Energies
*?Sp9PixP 2.2.3 Determination of Binding Energies and Chemical Shifts from Thermodynamic Data
f._FwD 2.3 Core Polarization
ovn)lIs 2.4 Final-State Multiplets in Rare-Earth Valence Bands
vpGeG 2.5 Vibrational Side Bands
7Bhi72&6 2.6 Core Levels of Adsorbed Molecules
K2glkGK 2.7 Quantitative Chemical Analysis from Core-Level Intensities
F(i@Gm=J] References
tOK lCc <ZV !fn 3. Charge-Excitation Final States: Satellites
P]4C/UDS-~ 3.1 Copper Dihalides; 3d Transition Metal Compounds
_ ecKX</Q 3.1.1 Characterization of a Satellite
v<z%\`y 3.1.2 Analysis of Charge-Transfer Satellites
{-(B 3.1.3 Non-local Screening
"3"9sIZ( 3.2 The 6-eV Satellite in Nickel
+)4_1i4"x 3.2.1 Resonance Photoemission
gL+8fX2G6 3.2.2 Satellites in Other Metals
C=6 Vd 3.3 The Gunnarsson-Sch6nhammer Theory
$6a55~h|( 3.4 Photoemission Signals and Narrow Bands in Metals
)(|+z' References
\)?[1b&[_ )o<rU[oD]C 4. Continuous Satellites and Plasmon Satellites: XPS Photoemission in Nearly Free Electron Systems
4epE!`z_& 4.1 Theory
>d&_e[j 4.1.1 General
/pvR-Id|6 4.1.2 Core-Line Shape
SoY= 4.1.3 Intrinsic Plasmons
A7!=`yA$ 4.1.4 Fxtrinsic FAectron Scattering: Plasmons and Background
n)(E 0h 4.1.5 The Total Photoelectron Spectrum
sILkTzsw 4.2 Experimental Results
BiQ7r=Dd. 4.2.1 The Core Line Without Plasmons
R30{/KK 4.2.2 Core-Level Spectra Including Plasmoas
U!L<v!$ 4.2.3 Valence-Band Spectra of the Simple Metals
3rEBG0cf] 4.2.4 Simple Metals: A General Comment
ROr..-[u 4.3 The Background Correction
P%v7(bqL4+ References
TixXA:Mf -o\r]24 5. Valence Orbitals in Simple Molecules and Insulating Solids
0^Vc,\P? 5.1 UPS Spectra of Monatomic Gases
Azun"F_f 5.2 Photoelectron Spectra of Diatomic Molecules
w6MEY"<L 5.3 Binding Energy of the H2 Molecule
6Hz45 5.4 Hydrides Isoelectronic with Noble Gases
0i2ZgOJ Neon (Ne)
!biq7f%6# Hydrogen Fluoride (HF)
=X?jId{ Water (H2O)
`Tx1?] Ammonia (NH3)
lZ5 lmsCU Methane (CH4)
x(nWyVB 5.5 Spectra of the Alkali HMides
Ldnw1xy 5.6 Transition Metal Dihalides
o:<gJzg 5.7 Hydrocarbons
oGi;S ="I 5.7.1 Guidelines for the Interpretation of Spectra from Free Molecules
6@TGa%:G 5.7.2 Linear Polymers
_h4{Sx 5.8 Insulating Solids with Valence d Electrons
72qbxPY13h 5.8.1 The NiO Problem
&y?L^Aq 5.8.2 Mort Insulation
Z_oBZs 5.8.3 The Metal-Insulator Transition;the Ratio of the Correlation Energy and the Bandwidth;Doping
D&f(h][hH? 5.8.4Band Structures of Transition Metal Compounds
_e<3 g9bj 5.9 High—Temperature Superconductors
<!#6c :(Q 5.9.1valence-Band Electronic Structure;Polycrystalline Samples
^[{\ZX 5.9.2 Dispersion Relations in High Temperature Superconductors;Single Crystals
Y4Hi<JWo 5.9.3 The Superconducting Gap
-z]v"gF?Px 5.9.4 Symmetry of the Order Parameter in the High-Temperature SuDerconductors
w\U
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?d)I!x,;; 5.10 The Fermi Liquid and the Luttinger Liquid
N'nI
^= 5.11 Adsorbed Molecules
`Z*k M VN 5.11.1 Outline
1/>#L6VAZ 5.11.2 CO on Metal Surfaces
:^+ aJ] References
N`7) 88>w **L . !/ 6.Photoemission of Valence Electrons froill Metallic Solids in the OHe-Electron Approximation
v:c_q]z#B 6.1 Theory of Photoemission:A Summary of the Three-Step Model
Hn%n>Bnl 6.2 Discussion of the Photocurrent
KXEDpr 6.2.1 Kinematics of Internal Photoemission in a Polycrystalline Sample
PSX-b)wb 6.2.2 Primary and Secondary Cones in the Photoemission from a Real Solid
;Ub;AqY 6.2.3 Angle-Integrated and Angle-Resolved Data Collection
VY)!bjW. 6.3 Photoemission from the Semi—infinite Crystal:The Inverse LEED Formalism
5UE5;yo 6.3.1 Band Structure Regime
E\2| 6.3.2 XPS Regime
)K2,h5zU 6.3.3 Surface Emission
@GzEhv 6.3.4 One-Step Calculations
<4,n6$E 6.4 Thermal Effects
LOf0_g/ 6.5 Dipole Selection Rules for Direct Optical Transitions
Z `FqC References
tL68
u[ u|l]8T9L 7.Band Structtire and Angular-Resolved Photoelectron Spectra
>'4Bq*5> 7.1 Free-Electron Final—State Model
|EuWzhNAO 7.2 Methods Employing Calculated Band Structures
;0Yeo"- 7.3 Methods for the Absolute Determination of the Crystal Momentum
.!T]sX_P 7.3.1 Triangulation or Energy Coincidence Method
;EZ$8| 7.3.2 Bragg Plane Method: Variation of External Emission Angle at Fixed Photon Frequency (Disappearance/Appearance Angle Method
Wpo:'?!(M^ 7.3.3 Bragg Plane Method: Variation of Photon Energy at Fixed Emission Angle (Symmetry Method)
,/n<Qg"` 7.3.4 The Surface Emission Method and Electron Damping
"G\OKt'Z 7.3.5 The Very-Low-Energy Electron Diffraction Method
8<}f:9/ 7.3.6 The Fermi Surface Method
;h>s=D,r 7.3.7 Intensities and Their Use in Band-Structure Determinations
5a1)`2V2M 7.3.8 Summary
VkCv`E 7.4 Experimental Band Structures
nlaJ 7.4.1 One- and Two-Dimensional Systems
G<9UL*HU 7.4.2 Three-Dimensional Solids: Metals and Semiconductors
trL:qD+{( 7..4.3UPS Band Structures and XPS Density of States
GQXN1R
7.5 A Comment
z}v6!u|iZu References
"Gx(-NH+ X(F2 5 8.Surface States, Surface Effects
` z<k7ig 8.1 Theoretical Considerations
]J\tosTi 8.2 Experimental Results on Surface States
)En*5-1 8.3 Quantum-Well States
YNCQPN\v`1 8.4 Surface Core-Level Shifts
au'Zjj/Ai5 References
y=) Cid 6]#pPk8[Z 9.Inverse Photoelectron Spectroscopy
>]?!c5= 9.1 Surface States
|) {)w` 9.2 Bulk Band Structures
N:Yjz^Jt 9.3 Adsorbed Molecules
GaMiu!|, References
]9]cef=h# i9?$BZQ[R 10. Spin-Polarized Photoelectron Spectroscopy
y21zaQ 10.1 General Description
e1ru#'z 10.2 Examples of Spin-Polarized Photoelectron Spectroscopy
Wh4`Iv\. 10.3 Magnetic Dichroism
W%@L7 xh References
ZW\}4q;[A 0U'g2F>{ 11. Photoelectron Diffraction
c`
^I% i 11.1 Examples
ndEW$?W, 11.2 Substrate Photoelectron Diffraction
;C,D1_20Z 11.3 Adsorbate Photoelectron Diffraction
Z'EXq.hk 11.4 Fermi Surface Scans
Jsf-t References
Ar4@7 9$F '*{8 Appendix
Qzbelt@Wx
A.1 Table of Binding Energies
KTX;x2r A.2 Surface and Bulk Brillouin Zones of the Three Low-Index Faces of a Face—Centered Cubic(fcc)Crystal Face
]i\C4* A.3 Compilation of Work Functions
>q0c!,Ay References
6|*em4 Index