光电子谱技术是研究原子、分子、固体和表面电子
结构的一种非常有效的手段。本书全面
系统地介绍了
光电子谱技术的
原理和应用,并简明讨论了逆光发射、自旋极化光发射和
光电子衍射等现象。本书是一本非常实用的光电子谱技术的专著,内容几乎覆盖了光电子研究的所有领域。其特点是紧密联系实验,并利用理论详细解释实验结果,达到理论和应用的有机结合。书中还收集了大量的实际
材料的光电子谱分析,同时给出了大量的实验数据,以便于读者的查阅。总之,该书既是一本很有价值的参考书,又可作为初学者的入门教材。
wb62($ Brxnl,%\ 作者在该领域做出了杰出的贡献。在第3版中,作者介绍了大量最新研究成果,并对光电子谱技术很多方面给出了有深刻见解的讨论。
w98M#GqV 6V$ )ym*F 读者对象:适用于凝聚态
物理学、材料物理学和光电子学等专业的高年级本科生、研究生和相关专业的科研人员。
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*e [* 1f+A_k/@ 目录
Z]uc *Ed 1. Introduction and Basic Principles
NB<8M!X/ 1.1 Historical Development
v CsE|eMP 1.2 The Electron Mean Free Path
y2+f)Xp_.C 1.3 Photoelectron Spectroscopy and Inverse Photoelectron Spectroscopy
ggPGKY-b= 1.4 Experimental Aspects
O$, 1.5 Very High Resolution
F#|y,<}< 1.6 The Theory of Photoemission
&v0]{)PO 1.6.1 Core-Level Photoemission
?J2A.x5`a 1.6.2 Valence-State Photoemission
@,oc%m 1.6.3 Three-Step and One-Step Considerations
wowf1j- 1.7 Deviations from the Simple Theory of Photoemission
%iNgHoH References
}^$#vJ(a7K K@e2%hk9x 2. Core Levels and Final States
EoutB Vm 2.1 Core-Level Binding Energies in Atoms and Molecules
GpTZp#~; 2.1.1 The Equivalent-Core Approximation
vmNo~clt\ 2.1.2 Chemical Shifts
Xbmsq,*] 2.2 Core-Level Binding Energies in Solids
\2+ngq) 2.2.1 The Born-Haber Cycle in Insulators
8!35
K 2.2.2 Theory of Binding Energies
rNhS\1- 2.2.3 Determination of Binding Energies and Chemical Shifts from Thermodynamic Data
l@SV!keQ 2.3 Core Polarization
`EgX# 2.4 Final-State Multiplets in Rare-Earth Valence Bands
QaLaw-lx 2.5 Vibrational Side Bands
OMk3\FV2Z 2.6 Core Levels of Adsorbed Molecules
Dn<3#V 2.7 Quantitative Chemical Analysis from Core-Level Intensities
EG^
rh; References
.s4vJKK0 H HX q_-V 3. Charge-Excitation Final States: Satellites
*2/qm:gB 3.1 Copper Dihalides; 3d Transition Metal Compounds
+fY@q,` 3.1.1 Characterization of a Satellite
DXD+,y\= 3.1.2 Analysis of Charge-Transfer Satellites
,k_ b-/ 3.1.3 Non-local Screening
;Egl8Vhr 3.2 The 6-eV Satellite in Nickel
dpE^BW v3 3.2.1 Resonance Photoemission
+pSo(e( 3.2.2 Satellites in Other Metals
yz0#0YG7 3.3 The Gunnarsson-Sch6nhammer Theory
ncadVheKt 3.4 Photoemission Signals and Narrow Bands in Metals
;\}dQsX References
E8PwA. i{N?Y0YQs0 4. Continuous Satellites and Plasmon Satellites: XPS Photoemission in Nearly Free Electron Systems
;yqHt!N 4.1 Theory
]6^S:K_" 4.1.1 General
2?LPr 4.1.2 Core-Line Shape
E3p$^['vx 4.1.3 Intrinsic Plasmons
}BW&1*M{ 4.1.4 Fxtrinsic FAectron Scattering: Plasmons and Background
S=S/]]e 4.1.5 The Total Photoelectron Spectrum
o_=4Ex
" 4.2 Experimental Results
VWt=9D; 4.2.1 The Core Line Without Plasmons
61QA<Wb 4.2.2 Core-Level Spectra Including Plasmoas
:Nf(:D8 4.2.3 Valence-Band Spectra of the Simple Metals
19[o XyFI 4.2.4 Simple Metals: A General Comment
oR`rs[Kj 4.3 The Background Correction
#s(ob `0| References
Ar~<l2,{r a5m[
N'kah 5. Valence Orbitals in Simple Molecules and Insulating Solids
QsPg4y3?D 5.1 UPS Spectra of Monatomic Gases
x(Uv>k~i} 5.2 Photoelectron Spectra of Diatomic Molecules
HZ!<dy3 5.3 Binding Energy of the H2 Molecule
Qt\:A!'jw 5.4 Hydrides Isoelectronic with Noble Gases
D&K9!z"] Neon (Ne)
Ok)f5")N % Hydrogen Fluoride (HF)
(qR;6l Water (H2O)
<i]-.>&J Ammonia (NH3)
1Hhr6T^) Methane (CH4)
)(.g~Q: 5.5 Spectra of the Alkali HMides
+8"8s 5.6 Transition Metal Dihalides
4gEw}WiP 5.7 Hydrocarbons
*!%n`BR ' 5.7.1 Guidelines for the Interpretation of Spectra from Free Molecules
,hJx3g5#n 5.7.2 Linear Polymers
(gE<`b 5.8 Insulating Solids with Valence d Electrons
7Q'u>o 5.8.1 The NiO Problem
3&E@#I^], 5.8.2 Mort Insulation
*C|*{! 5.8.3 The Metal-Insulator Transition;the Ratio of the Correlation Energy and the Bandwidth;Doping
0n4( Rj|}2 5.8.4Band Structures of Transition Metal Compounds
R$IsP,Uw 5.9 High—Temperature Superconductors
O5:U2o- 5.9.1valence-Band Electronic Structure;Polycrystalline Samples
SJc*Rl> 5.9.2 Dispersion Relations in High Temperature Superconductors;Single Crystals
!"/"Mqs3$ 5.9.3 The Superconducting Gap
/W
f.Gt9[ 5.9.4 Symmetry of the Order Parameter in the High-Temperature SuDerconductors
RWu<
dY#ym 5.9.5 Core—Level Shifts
{C?$osrr 5.10 The Fermi Liquid and the Luttinger Liquid
t:oq't 5.11 Adsorbed Molecules
p|qLr9\A 5.11.1 Outline
hxJKYU^%m 5.11.2 CO on Metal Surfaces
#~m^RoE References
N&G(`] Q A~F
6.Photoemission of Valence Electrons froill Metallic Solids in the OHe-Electron Approximation
u f<%!=e 6.1 Theory of Photoemission:A Summary of the Three-Step Model
bhg6p$411 6.2 Discussion of the Photocurrent
QCDica `+* 6.2.1 Kinematics of Internal Photoemission in a Polycrystalline Sample
Je"XIhBr 6.2.2 Primary and Secondary Cones in the Photoemission from a Real Solid
&\5bo=5V 6.2.3 Angle-Integrated and Angle-Resolved Data Collection
FncP,F$8
6.3 Photoemission from the Semi—infinite Crystal:The Inverse LEED Formalism
j5n"LC+oz 6.3.1 Band Structure Regime
{Z!t:'x8 6.3.2 XPS Regime
#/9Y}2G|] 6.3.3 Surface Emission
<jFov`^ 6.3.4 One-Step Calculations
*yZta:(w-W 6.4 Thermal Effects
dpge:Qhr 6.5 Dipole Selection Rules for Direct Optical Transitions
Kx[+$Qt References
qKeR}&b sGiK
S,.K 7.Band Structtire and Angular-Resolved Photoelectron Spectra
Y>E` 7n 7.1 Free-Electron Final—State Model
6v}q @z 7.2 Methods Employing Calculated Band Structures
DBu8}2R 7.3 Methods for the Absolute Determination of the Crystal Momentum
*GhV1# < 7.3.1 Triangulation or Energy Coincidence Method
&F;bg 7.3.2 Bragg Plane Method: Variation of External Emission Angle at Fixed Photon Frequency (Disappearance/Appearance Angle Method
3*7 klu 7.3.3 Bragg Plane Method: Variation of Photon Energy at Fixed Emission Angle (Symmetry Method)
8In~qf 7.3.4 The Surface Emission Method and Electron Damping
@kT@IQkri 7.3.5 The Very-Low-Energy Electron Diffraction Method
Xa"I 7.3.6 The Fermi Surface Method
8{icY|:MTN 7.3.7 Intensities and Their Use in Band-Structure Determinations
GqP02P'2 7.3.8 Summary
|,TBP@ 7.4 Experimental Band Structures
|Q%nnN 7.4.1 One- and Two-Dimensional Systems
aAd1[?& 7.4.2 Three-Dimensional Solids: Metals and Semiconductors
KdTWi;mV2- 7..4.3UPS Band Structures and XPS Density of States
1B 0[dK2N 7.5 A Comment
/UR;,ts References
09Q5gal bq5we*"V 8.Surface States, Surface Effects
VggSDb 8.1 Theoretical Considerations
V=>]&95-f 8.2 Experimental Results on Surface States
NVom6K 8.3 Quantum-Well States
siV]NI':| 8.4 Surface Core-Level Shifts
Y>2#9LA References
AEFd,;GF oj?y_0}:^ 9.Inverse Photoelectron Spectroscopy
|Zo36@s 9.1 Surface States
I&^hG\D 9.2 Bulk Band Structures
]gA2.,)}D 9.3 Adsorbed Molecules
x
FvKjO) References
G_k_qP^: '['x'G50 10. Spin-Polarized Photoelectron Spectroscopy
]_!NmB_3 10.1 General Description
=yJV8%pa 10.2 Examples of Spin-Polarized Photoelectron Spectroscopy
d,'gh4C 10.3 Magnetic Dichroism
xA*6Z)Y References
&[PA?#I` zqXDD; w3 11. Photoelectron Diffraction
x>J(3I5_b 11.1 Examples
9RK.+2 11.2 Substrate Photoelectron Diffraction
NOAz"m+o 11.3 Adsorbate Photoelectron Diffraction
(2 hI 11.4 Fermi Surface Scans
vMJ_n=Vf References
GbkDs- j(pe6 Appendix
VYH
$em6 A.1 Table of Binding Energies
OwDwa~ A.2 Surface and Bulk Brillouin Zones of the Three Low-Index Faces of a Face—Centered Cubic(fcc)Crystal Face
d7Cs a
c A.3 Compilation of Work Functions
BuitM|k' References
3Zp q# Index