光电子谱技术是研究原子、分子、固体和表面电子
结构的一种非常有效的手段。本书全面
系统地介绍了
光电子谱技术的
原理和应用,并简明讨论了逆光发射、自旋极化光发射和
光电子衍射等现象。本书是一本非常实用的光电子谱技术的专著,内容几乎覆盖了光电子研究的所有领域。其特点是紧密联系实验,并利用理论详细解释实验结果,达到理论和应用的有机结合。书中还收集了大量的实际
材料的光电子谱分析,同时给出了大量的实验数据,以便于读者的查阅。总之,该书既是一本很有价值的参考书,又可作为初学者的入门教材。
MUB37
$o"g73`3 作者在该领域做出了杰出的贡献。在第3版中,作者介绍了大量最新研究成果,并对光电子谱技术很多方面给出了有深刻见解的讨论。
N ocFvF7\ 4#7Umj 读者对象:适用于凝聚态
物理学、材料物理学和光电子学等专业的高年级本科生、研究生和相关专业的科研人员。
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5uttv:@= _Z.cMYN 目录
;iQp7aW{$ 1. Introduction and Basic Principles
GG+5/hU 1.1 Historical Development
Z\' wm' 1.2 The Electron Mean Free Path
{>h97}P 1.3 Photoelectron Spectroscopy and Inverse Photoelectron Spectroscopy
}PZ=`w*O 1.4 Experimental Aspects
'W(xgOP1 1.5 Very High Resolution
!UcOl0"6 1.6 The Theory of Photoemission
4w;~4#ZPp 1.6.1 Core-Level Photoemission
T
.hb#oO 1.6.2 Valence-State Photoemission
$kl$D"*0 1.6.3 Three-Step and One-Step Considerations
%Hwbw],kl8 1.7 Deviations from the Simple Theory of Photoemission
ZV(
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qv uxhz F OX^3Q:Z= 2. Core Levels and Final States
A9;0y jae 2.1 Core-Level Binding Energies in Atoms and Molecules
~#Aa Ldq 2.1.1 The Equivalent-Core Approximation
i.M2E$b| 2.1.2 Chemical Shifts
tr=@+WHp 2.2 Core-Level Binding Energies in Solids
yd*3)6= 2.2.1 The Born-Haber Cycle in Insulators
Sr"/- 2.2.2 Theory of Binding Energies
M(2`2-/xh 2.2.3 Determination of Binding Energies and Chemical Shifts from Thermodynamic Data
K:_($X] 2.3 Core Polarization
lhxdx 2.4 Final-State Multiplets in Rare-Earth Valence Bands
K}K)`bifw 2.5 Vibrational Side Bands
vI|As+`$d 2.6 Core Levels of Adsorbed Molecules
nvH|Ngg Q 2.7 Quantitative Chemical Analysis from Core-Level Intensities
> 0T
Za References
dhtb?n{
'F7VM?HBfg 3. Charge-Excitation Final States: Satellites
eT-9 3.1 Copper Dihalides; 3d Transition Metal Compounds
\igaQ\~ 3.1.1 Characterization of a Satellite
gc,Ps 3.1.2 Analysis of Charge-Transfer Satellites
M _ (2sq 3.1.3 Non-local Screening
:1MMa6 3.2 The 6-eV Satellite in Nickel
c3W
BALdh 3.2.1 Resonance Photoemission
>|nt2 3.2.2 Satellites in Other Metals
y
1nU{Sc@ 3.3 The Gunnarsson-Sch6nhammer Theory
_Ex|f5+ 3.4 Photoemission Signals and Narrow Bands in Metals
M BVOfEMj References
n| C|& 'Sa!5h 4. Continuous Satellites and Plasmon Satellites: XPS Photoemission in Nearly Free Electron Systems
T VeJ6 4.1 Theory
SQE`
U 4.1.1 General
aS/`A 4.1.2 Core-Line Shape
Y 1y E 4.1.3 Intrinsic Plasmons
3I*uV!notJ 4.1.4 Fxtrinsic FAectron Scattering: Plasmons and Background
q~O>a0f0 4.1.5 The Total Photoelectron Spectrum
v20~^gKo=m 4.2 Experimental Results
~6HDW 4.2.1 The Core Line Without Plasmons
sUciFAb 4.2.2 Core-Level Spectra Including Plasmoas
(}jL_E 4.2.3 Valence-Band Spectra of the Simple Metals
U&Ab#m; 4.2.4 Simple Metals: A General Comment
?d5h9}B 4.3 The Background Correction
hVf^ References
>qpqQ;
bm lD3)TAW@o 5. Valence Orbitals in Simple Molecules and Insulating Solids
> UWStzH< 5.1 UPS Spectra of Monatomic Gases
wv^b_DR 5.2 Photoelectron Spectra of Diatomic Molecules
@|=UrKA N 5.3 Binding Energy of the H2 Molecule
!
Rvn'|! 5.4 Hydrides Isoelectronic with Noble Gases
1R^4C8*B Neon (Ne)
X+at%L= Hydrogen Fluoride (HF)
=UUd8,C/ Water (H2O)
aTClw<6} Ammonia (NH3)
L|J~9FM Methane (CH4)
EneAX&SG 5.5 Spectra of the Alkali HMides
m^A]+G#/ 5.6 Transition Metal Dihalides
\ 3G*j` 5.7 Hydrocarbons
ev"M;"y 5.7.1 Guidelines for the Interpretation of Spectra from Free Molecules
VVLIeJ(*XT 5.7.2 Linear Polymers
N7pt:G2~% 5.8 Insulating Solids with Valence d Electrons
Q!]IG;3Sx| 5.8.1 The NiO Problem
r--;yEjWE 5.8.2 Mort Insulation
(#z;(EN0t 5.8.3 The Metal-Insulator Transition;the Ratio of the Correlation Energy and the Bandwidth;Doping
\u8,!) 4i 5.8.4Band Structures of Transition Metal Compounds
l5HWZs^ 5.9 High—Temperature Superconductors
_[JkJwPTx 5.9.1valence-Band Electronic Structure;Polycrystalline Samples
3agNB F2 5.9.2 Dispersion Relations in High Temperature Superconductors;Single Crystals
$iHoOYx]< 5.9.3 The Superconducting Gap
:x+ig5 5.9.4 Symmetry of the Order Parameter in the High-Temperature SuDerconductors
>%h7dC3h 5.9.5 Core—Level Shifts
j{"[Ec 5.10 The Fermi Liquid and the Luttinger Liquid
^ $wJi9D6 5.11 Adsorbed Molecules
v:A:37#I 5.11.1 Outline
Fx5ZwT
t 5.11.2 CO on Metal Surfaces
Z(UD9wY5m References
P&\X`ZUA I%i:)6Un-y 6.Photoemission of Valence Electrons froill Metallic Solids in the OHe-Electron Approximation
`M)E* G 6.1 Theory of Photoemission:A Summary of the Three-Step Model
Y}/c
N\ 6.2 Discussion of the Photocurrent
|z+9km7, 6.2.1 Kinematics of Internal Photoemission in a Polycrystalline Sample
xE1rxPuq)d 6.2.2 Primary and Secondary Cones in the Photoemission from a Real Solid
df
?eL2v 6.2.3 Angle-Integrated and Angle-Resolved Data Collection
C fSl
54 6.3 Photoemission from the Semi—infinite Crystal:The Inverse LEED Formalism
-5xCQJ[ 6.3.1 Band Structure Regime
<A{y($ 6.3.2 XPS Regime
"&Mou 6.3.3 Surface Emission
6Hn)pD#U 6.3.4 One-Step Calculations
B-dlm8gX
6.4 Thermal Effects
F"=Hp4-C 6.5 Dipole Selection Rules for Direct Optical Transitions
>HIt}Zh References
}!=U^A) >-zkB)5<,# 7.Band Structtire and Angular-Resolved Photoelectron Spectra
@?d?e+B 7.1 Free-Electron Final—State Model
ngLJ@TP- 7.2 Methods Employing Calculated Band Structures
x
^[F]YU 7.3 Methods for the Absolute Determination of the Crystal Momentum
yLB~P7K 7.3.1 Triangulation or Energy Coincidence Method
3I\m,Ob 7.3.2 Bragg Plane Method: Variation of External Emission Angle at Fixed Photon Frequency (Disappearance/Appearance Angle Method
#s{aulx 7.3.3 Bragg Plane Method: Variation of Photon Energy at Fixed Emission Angle (Symmetry Method)
pw;r 25 7.3.4 The Surface Emission Method and Electron Damping
*/Cj$KY70 7.3.5 The Very-Low-Energy Electron Diffraction Method
esteFLm`6 7.3.6 The Fermi Surface Method
| lE-&a$xd 7.3.7 Intensities and Their Use in Band-Structure Determinations
&SrGh$:X 7.3.8 Summary
CrO`=\ 7.4 Experimental Band Structures
]4GZ'&m} 7.4.1 One- and Two-Dimensional Systems
9t}J|09i 7.4.2 Three-Dimensional Solids: Metals and Semiconductors
wibwyzo 7..4.3UPS Band Structures and XPS Density of States
rg*^w! 7.5 A Comment
D2)i3vFB References
{NV:|M ! ssT@<Tk^4 8.Surface States, Surface Effects
'+6<U[ L 8.1 Theoretical Considerations
Th/{x
h 8.2 Experimental Results on Surface States
|=u96G~N 8.3 Quantum-Well States
)^";BVY 8.4 Surface Core-Level Shifts
Vpw[B.v References
on_H6Y@B52 T*R{L 9.Inverse Photoelectron Spectroscopy
44j,,k 9.1 Surface States
,m3":{G:t. 9.2 Bulk Band Structures
o~k;D{Snr 9.3 Adsorbed Molecules
;b| References
Fn> <q: .8x@IWJD 10. Spin-Polarized Photoelectron Spectroscopy
]K*GSU 10.1 General Description
sNf
+ lga0 10.2 Examples of Spin-Polarized Photoelectron Spectroscopy
e z+yP,.# 10.3 Magnetic Dichroism
19) !$Hl References
Y!it!9 c(CJ{>F% 11. Photoelectron Diffraction
EZ `}*Yrd 11.1 Examples
DiR'p`b~ 11.2 Substrate Photoelectron Diffraction
~M; gM]r; 11.3 Adsorbate Photoelectron Diffraction
N"K\ick6J 11.4 Fermi Surface Scans
IW mHp] References
>HX)MwAP Gn[ *?=Vy Appendix
@'Q%Jc( A.1 Table of Binding Energies
E^82==R A.2 Surface and Bulk Brillouin Zones of the Three Low-Index Faces of a Face—Centered Cubic(fcc)Crystal Face
9':/Sab:7v A.3 Compilation of Work Functions
3@'lIV
?,q References
G\):2Qz!| Index