光电子谱技术是研究原子、分子、固体和表面电子
结构的一种非常有效的手段。本书全面
系统地介绍了
光电子谱技术的
原理和应用,并简明讨论了逆光发射、自旋极化光发射和
光电子衍射等现象。本书是一本非常实用的光电子谱技术的专著,内容几乎覆盖了光电子研究的所有领域。其特点是紧密联系实验,并利用理论详细解释实验结果,达到理论和应用的有机结合。书中还收集了大量的实际
材料的光电子谱分析,同时给出了大量的实验数据,以便于读者的查阅。总之,该书既是一本很有价值的参考书,又可作为初学者的入门教材。
#Kh`ATme }F3Z~ 作者在该领域做出了杰出的贡献。在第3版中,作者介绍了大量最新研究成果,并对光电子谱技术很多方面给出了有深刻见解的讨论。
z?gJHN< &c\8`# 6 读者对象:适用于凝聚态
物理学、材料物理学和光电子学等专业的高年级本科生、研究生和相关专业的科研人员。
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8WyG49eic 4B> l|% 目录
~}M{[6! 1. Introduction and Basic Principles
@eMyq1ZU 1.1 Historical Development
-!}1{ 1.2 The Electron Mean Free Path
X:e'@]Z)? 1.3 Photoelectron Spectroscopy and Inverse Photoelectron Spectroscopy
2xnOWW 1.4 Experimental Aspects
ZHF@k'vm/9 1.5 Very High Resolution
Mr1pRIYMd 1.6 The Theory of Photoemission
6@$[x* V 1.6.1 Core-Level Photoemission
l%U9g 1.6.2 Valence-State Photoemission
Z6*RIdD> 1.6.3 Three-Step and One-Step Considerations
|/(5GX,X 1.7 Deviations from the Simple Theory of Photoemission
eU12*( References
/J6CSk EP8LJzd" 2. Core Levels and Final States
1rKR=To 2.1 Core-Level Binding Energies in Atoms and Molecules
asJYGqdF 2.1.1 The Equivalent-Core Approximation
<T}#>xHs3 2.1.2 Chemical Shifts
O@$hG8: 2.2 Core-Level Binding Energies in Solids
tT
v@8f 2.2.1 The Born-Haber Cycle in Insulators
\.{JS>! 2.2.2 Theory of Binding Energies
_AO0:& 2.2.3 Determination of Binding Energies and Chemical Shifts from Thermodynamic Data
c49#aNR 2.3 Core Polarization
[6Wr
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>:xnjEsi$/ 2.5 Vibrational Side Bands
F0!r9U(( 2.6 Core Levels of Adsorbed Molecules
F?dTCa 2.7 Quantitative Chemical Analysis from Core-Level Intensities
kQb0pfYs References
q3[LnmH 8%NX)hZyq} 3. Charge-Excitation Final States: Satellites
hh?'tb{ 3.1 Copper Dihalides; 3d Transition Metal Compounds
=?2y
<B 3.1.1 Characterization of a Satellite
cn#a/Hx 3.1.2 Analysis of Charge-Transfer Satellites
*H$nydQ: 3.1.3 Non-local Screening
/qCYNwWH9 3.2 The 6-eV Satellite in Nickel
H{V-C_ 3.2.1 Resonance Photoemission
m0edkt-x 3.2.2 Satellites in Other Metals
hw7_8pAbh 3.3 The Gunnarsson-Sch6nhammer Theory
lAGxE-B^a" 3.4 Photoemission Signals and Narrow Bands in Metals
{NFeX'5bP References
226s:\d G'epsD,.bX 4. Continuous Satellites and Plasmon Satellites: XPS Photoemission in Nearly Free Electron Systems
lt*k(JD 4.1 Theory
7q?YdAUz 4.1.1 General
*K)v&}uw 4.1.2 Core-Line Shape
l&rDa=m.J 4.1.3 Intrinsic Plasmons
<hea%6 4.1.4 Fxtrinsic FAectron Scattering: Plasmons and Background
yO6i "3 4.1.5 The Total Photoelectron Spectrum
~U1iB 4.2 Experimental Results
<Kh\i'8 4.2.1 The Core Line Without Plasmons
vW_A.iI"e 4.2.2 Core-Level Spectra Including Plasmoas
4EpzCaEZ 4.2.3 Valence-Band Spectra of the Simple Metals
Cam}:'a/` 4.2.4 Simple Metals: A General Comment
Cb13 Qz 4.3 The Background Correction
Ntqc=z References
pFK
|4u Z 0:2x(x9 5. Valence Orbitals in Simple Molecules and Insulating Solids
8x{vgx @M 5.1 UPS Spectra of Monatomic Gases
J.&q[ 5.2 Photoelectron Spectra of Diatomic Molecules
OBl8kH(b> 5.3 Binding Energy of the H2 Molecule
MJb = +L 5.4 Hydrides Isoelectronic with Noble Gases
{,
|"Rpd Neon (Ne)
QA3l:D}u Hydrogen Fluoride (HF)
Z^|C~lp;n Water (H2O)
*"5a5.`%, Ammonia (NH3)
R*y[/Aw Methane (CH4)
rNAu@B 5.5 Spectra of the Alkali HMides
z>{KeX: 5.6 Transition Metal Dihalides
EH3G|3^xz 5.7 Hydrocarbons
)k1,oUx 5.7.1 Guidelines for the Interpretation of Spectra from Free Molecules
H>]z=w~ 5.7.2 Linear Polymers
|x4yPYBL 5.8 Insulating Solids with Valence d Electrons
sHuz10 5.8.1 The NiO Problem
KFhn}C3
i 5.8.2 Mort Insulation
D7.P 5.8.3 The Metal-Insulator Transition;the Ratio of the Correlation Energy and the Bandwidth;Doping
K8Y/XEK 5.8.4Band Structures of Transition Metal Compounds
2%8Y-o? 5.9 High—Temperature Superconductors
IX(yajc[~M 5.9.1valence-Band Electronic Structure;Polycrystalline Samples
I5A^/=bf& 5.9.2 Dispersion Relations in High Temperature Superconductors;Single Crystals
{q)B@#p 5.9.3 The Superconducting Gap
g?VME]: 5.9.4 Symmetry of the Order Parameter in the High-Temperature SuDerconductors
E
oR(/*' 5.9.5 Core—Level Shifts
[w/t 5.10 The Fermi Liquid and the Luttinger Liquid
Z)A+ wM 5.11 Adsorbed Molecules
rrWk&;? 5.11.1 Outline
##_Za6/n 5.11.2 CO on Metal Surfaces
M;Rw]M References
gdK/:%u3 "6dbRo5% 6.Photoemission of Valence Electrons froill Metallic Solids in the OHe-Electron Approximation
WK}+f4tdW[ 6.1 Theory of Photoemission:A Summary of the Three-Step Model
/RC!Yi 6.2 Discussion of the Photocurrent
{|h"/ 6.2.1 Kinematics of Internal Photoemission in a Polycrystalline Sample
"k|`xn 6.2.2 Primary and Secondary Cones in the Photoemission from a Real Solid
h6e$$-_ 6.2.3 Angle-Integrated and Angle-Resolved Data Collection
$te,\$&} 6.3 Photoemission from the Semi—infinite Crystal:The Inverse LEED Formalism
G7;}309s 6.3.1 Band Structure Regime
lnWiE}F 6.3.2 XPS Regime
F"H!CJJu& 6.3.3 Surface Emission
w2+]C&B* 6.3.4 One-Step Calculations
aTm.10{^ 6.4 Thermal Effects
j*u9+. 6.5 Dipole Selection Rules for Direct Optical Transitions
W~F/ZrT3A References
\,!q[nC SU'9+=_$ 7.Band Structtire and Angular-Resolved Photoelectron Spectra
KaE;4gwM 7.1 Free-Electron Final—State Model
*`-29eR"8 7.2 Methods Employing Calculated Band Structures
}?J5!X 7.3 Methods for the Absolute Determination of the Crystal Momentum
BznA)EK?@ 7.3.1 Triangulation or Energy Coincidence Method
y7-:l u$9 7.3.2 Bragg Plane Method: Variation of External Emission Angle at Fixed Photon Frequency (Disappearance/Appearance Angle Method
uW~,H}E 7.3.3 Bragg Plane Method: Variation of Photon Energy at Fixed Emission Angle (Symmetry Method)
4.B*B3 7.3.4 The Surface Emission Method and Electron Damping
;cn.s, 7.3.5 The Very-Low-Energy Electron Diffraction Method
ls\E%d 7.3.6 The Fermi Surface Method
t)Q@sKT6 7.3.7 Intensities and Their Use in Band-Structure Determinations
.b`P! 7.3.8 Summary
bDS1'Ce 7.4 Experimental Band Structures
]~Vu-@
/} 7.4.1 One- and Two-Dimensional Systems
'F?Znd2L 7.4.2 Three-Dimensional Solids: Metals and Semiconductors
Qf>Pb$c$U 7..4.3UPS Band Structures and XPS Density of States
B9Q.s 7.5 A Comment
&jZ|@K? References
Gy6qLM ]3,.g)U*m 8.Surface States, Surface Effects
9*+0j2uhQ 8.1 Theoretical Considerations
fsc~$^.~\ 8.2 Experimental Results on Surface States
z~e~K`S 8.3 Quantum-Well States
@nX2*j*u 8.4 Surface Core-Level Shifts
<lmJa# References
niEEm`"
tW:/R@@ 9.Inverse Photoelectron Spectroscopy
wv.Ulrpx. 9.1 Surface States
K}<!{/fi) 9.2 Bulk Band Structures
#K1BJ#KUt 9.3 Adsorbed Molecules
Y0yO`W4 References
x<j"DS}S)D 50GYL5)q 10. Spin-Polarized Photoelectron Spectroscopy
kqvJ&7 10.1 General Description
u%1k 10.2 Examples of Spin-Polarized Photoelectron Spectroscopy
o-=d|dWG 10.3 Magnetic Dichroism
vZeYp References
@Du}
EKd3$(^ 11. Photoelectron Diffraction
a!y,!EB+Qu 11.1 Examples
Wj j2J8B 11.2 Substrate Photoelectron Diffraction
,Q=)$ `% 11.3 Adsorbate Photoelectron Diffraction
JM-ce8U 11.4 Fermi Surface Scans
bjPbl2K References
Rs F3#H b({Nf,(a2
Appendix
e9`uD|KAS| A.1 Table of Binding Energies
"-QRkif A.2 Surface and Bulk Brillouin Zones of the Three Low-Index Faces of a Face—Centered Cubic(fcc)Crystal Face
r d6F"W A.3 Compilation of Work Functions
U 'CfP9= References
f >)Tq' Index