光电子谱技术是研究原子、分子、固体和表面电子
结构的一种非常有效的手段。本书全面
系统地介绍了
光电子谱技术的
原理和应用,并简明讨论了逆光发射、自旋极化光发射和
光电子衍射等现象。本书是一本非常实用的光电子谱技术的专著,内容几乎覆盖了光电子研究的所有领域。其特点是紧密联系实验,并利用理论详细解释实验结果,达到理论和应用的有机结合。书中还收集了大量的实际
材料的光电子谱分析,同时给出了大量的实验数据,以便于读者的查阅。总之,该书既是一本很有价值的参考书,又可作为初学者的入门教材。
&H$
3`"p5u )Q9m,/F 作者在该领域做出了杰出的贡献。在第3版中,作者介绍了大量最新研究成果,并对光电子谱技术很多方面给出了有深刻见解的讨论。
K#H}=Y A z:-a7_ 读者对象:适用于凝聚态
物理学、材料物理学和光电子学等专业的高年级本科生、研究生和相关专业的科研人员。
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;E>5<[aa ]c]rIOTN 目录
e p~3e5 1. Introduction and Basic Principles
-v.\CtpHv 1.1 Historical Development
34k<7X`I 1.2 The Electron Mean Free Path
B~QX{ 1.3 Photoelectron Spectroscopy and Inverse Photoelectron Spectroscopy
b|U&{I>TH 1.4 Experimental Aspects
CdgZq\ 1.5 Very High Resolution
2ikY.Xi6 1.6 The Theory of Photoemission
ce th )Xm 1.6.1 Core-Level Photoemission
_"_ W KlN 1.6.2 Valence-State Photoemission
_"
W<> 1.6.3 Three-Step and One-Step Considerations
"-GjwB 1.7 Deviations from the Simple Theory of Photoemission
GY,l&.& References
'uS!rKkQlu *`OgwMr)M 2. Core Levels and Final States
JUXIE y^ 2.1 Core-Level Binding Energies in Atoms and Molecules
n#t{3qzpD 2.1.1 The Equivalent-Core Approximation
MEMD8:[' 2.1.2 Chemical Shifts
Nl3x
BM% 2.2 Core-Level Binding Energies in Solids
8rwkux > 2.2.1 The Born-Haber Cycle in Insulators
4wh_iO 2.2.2 Theory of Binding Energies
sE@t$'= 2.2.3 Determination of Binding Energies and Chemical Shifts from Thermodynamic Data
&cztUM( 2.3 Core Polarization
j@1cllJkh 2.4 Final-State Multiplets in Rare-Earth Valence Bands
["|AD,$% 2.5 Vibrational Side Bands
q+f]E&': 2.6 Core Levels of Adsorbed Molecules
yG|^-O}L 2.7 Quantitative Chemical Analysis from Core-Level Intensities
S%gb1's References
i <0H W J/S 47J~ 3. Charge-Excitation Final States: Satellites
xO)vn\uJ 3.1 Copper Dihalides; 3d Transition Metal Compounds
jjbBv~vs 3.1.1 Characterization of a Satellite
LWE[]1= 3.1.2 Analysis of Charge-Transfer Satellites
H6(kxpOI\ 3.1.3 Non-local Screening
^N}zePy0 3.2 The 6-eV Satellite in Nickel
B2t.;uz(, 3.2.1 Resonance Photoemission
ga&l.:lo 3.2.2 Satellites in Other Metals
:=vB|Ch:~ 3.3 The Gunnarsson-Sch6nhammer Theory
JF!?i6V 3.4 Photoemission Signals and Narrow Bands in Metals
*5Upb,** References
Ry>c]\a] z2Sp 4. Continuous Satellites and Plasmon Satellites: XPS Photoemission in Nearly Free Electron Systems
7^,C=2
4.1 Theory
ktLXL;~X 4.1.1 General
+^tq?PfE 4.1.2 Core-Line Shape
yL/EIN 4.1.3 Intrinsic Plasmons
>yFEUD: 4.1.4 Fxtrinsic FAectron Scattering: Plasmons and Background
d2lOx|jt 4.1.5 The Total Photoelectron Spectrum
meunAEe 4.2 Experimental Results
k%-_z}:3V 4.2.1 The Core Line Without Plasmons
AujvKQ( 4.2.2 Core-Level Spectra Including Plasmoas
%"^$$$6% 4.2.3 Valence-Band Spectra of the Simple Metals
uU(G &:@ 4.2.4 Simple Metals: A General Comment
U;Z6o1G 4.3 The Background Correction
U">J$M@ References
RK?b/9y 54~`8f 5. Valence Orbitals in Simple Molecules and Insulating Solids
ModwJ
w 5.1 UPS Spectra of Monatomic Gases
<![tn#_ 5.2 Photoelectron Spectra of Diatomic Molecules
jqxeON 5.3 Binding Energy of the H2 Molecule
WmU4~. 5.4 Hydrides Isoelectronic with Noble Gases
dA>=#/" Neon (Ne)
:q=u+h_ Hydrogen Fluoride (HF)
(\m4o
Water (H2O)
f1MKYM%^x Ammonia (NH3)
l'=H,8LfA Methane (CH4)
eq.K77El{J 5.5 Spectra of the Alkali HMides
*Wk y# 5.6 Transition Metal Dihalides
*KNj5>6= 5.7 Hydrocarbons
gX<"-,5jc 5.7.1 Guidelines for the Interpretation of Spectra from Free Molecules
Sx)b~ * 5.7.2 Linear Polymers
yoa"21E$ 5.8 Insulating Solids with Valence d Electrons
`<&RZB2 5.8.1 The NiO Problem
Jj+|>(P 5.8.2 Mort Insulation
usEdp 5.8.3 The Metal-Insulator Transition;the Ratio of the Correlation Energy and the Bandwidth;Doping
cF!ygz// 5.8.4Band Structures of Transition Metal Compounds
Nq'Cuwsp 5.9 High—Temperature Superconductors
h(]aP<49L 5.9.1valence-Band Electronic Structure;Polycrystalline Samples
2[f8"'lUQ 5.9.2 Dispersion Relations in High Temperature Superconductors;Single Crystals
H59}d
oKH 5.9.3 The Superconducting Gap
+c4]}9f! 5.9.4 Symmetry of the Order Parameter in the High-Temperature SuDerconductors
y<mmv~= 5.9.5 Core—Level Shifts
}~pT
saw 5.10 The Fermi Liquid and the Luttinger Liquid
e!
V`cg0 5.11 Adsorbed Molecules
~]f+ 5.11.1 Outline
y1R53u`;L 5.11.2 CO on Metal Surfaces
qN((Xz+AZE References
3wZA,Z
{~NiGHY 6.Photoemission of Valence Electrons froill Metallic Solids in the OHe-Electron Approximation
S@i*+&Ot 6.1 Theory of Photoemission:A Summary of the Three-Step Model
oC0K!{R* 6.2 Discussion of the Photocurrent
L,#ij!txS 6.2.1 Kinematics of Internal Photoemission in a Polycrystalline Sample
~EJVlji 6.2.2 Primary and Secondary Cones in the Photoemission from a Real Solid
gwE#,OY* 6.2.3 Angle-Integrated and Angle-Resolved Data Collection
!G E-5 \* 6.3 Photoemission from the Semi—infinite Crystal:The Inverse LEED Formalism
X,VOKj.% 6.3.1 Band Structure Regime
zf-)c1$*r 6.3.2 XPS Regime
gyi<ot; 6.3.3 Surface Emission
_kUf[& 6.3.4 One-Step Calculations
ozN#LIM>P 6.4 Thermal Effects
>DX\^86x 6.5 Dipole Selection Rules for Direct Optical Transitions
#T<<{ RA References
d|5V"U]W; ,)%al76E 7.Band Structtire and Angular-Resolved Photoelectron Spectra
Z)E[Bv= 7.1 Free-Electron Final—State Model
ZuZe8& 7.2 Methods Employing Calculated Band Structures
%oVoE2T{@ 7.3 Methods for the Absolute Determination of the Crystal Momentum
bOR1V\Jr$q 7.3.1 Triangulation or Energy Coincidence Method
gP=(2EVE 7.3.2 Bragg Plane Method: Variation of External Emission Angle at Fixed Photon Frequency (Disappearance/Appearance Angle Method
fNb2>1 7.3.3 Bragg Plane Method: Variation of Photon Energy at Fixed Emission Angle (Symmetry Method)
L=Cm0q 3v 7.3.4 The Surface Emission Method and Electron Damping
H9'Y` -r 7.3.5 The Very-Low-Energy Electron Diffraction Method
gBM6{48GF 7.3.6 The Fermi Surface Method
;Zfglid 7.3.7 Intensities and Their Use in Band-Structure Determinations
7"}<J7"}) 7.3.8 Summary
=7%1] 7.4 Experimental Band Structures
I2G4j/c=z 7.4.1 One- and Two-Dimensional Systems
Jlgo@?Lc 7.4.2 Three-Dimensional Solids: Metals and Semiconductors
SF$'$6x} 7..4.3UPS Band Structures and XPS Density of States
Vk%[N> 7.5 A Comment
QC@nRy8% References
yVA<-PlS< )Los\6PRn 8.Surface States, Surface Effects
bvdAOvxChW 8.1 Theoretical Considerations
?kBi9^)N4 8.2 Experimental Results on Surface States
.xJW=G{/ 8.3 Quantum-Well States
cQ kH4>C~ 8.4 Surface Core-Level Shifts
#$q~ZKB References
Gvg)@VNr ,\*PpcU 9.Inverse Photoelectron Spectroscopy
m$nT#@l5bH 9.1 Surface States
OO)m{5r,{ 9.2 Bulk Band Structures
kmHIU}Z 9.3 Adsorbed Molecules
:4 9ttJl References
#H9J/k_ E"LSM]^^<f 10. Spin-Polarized Photoelectron Spectroscopy
ut26sg{s( 10.1 General Description
rv`kP"I 10.2 Examples of Spin-Polarized Photoelectron Spectroscopy
pfd||Z 10.3 Magnetic Dichroism
#1-y[w/ References
3GMRH;/w r$3{1HXc 11. Photoelectron Diffraction
o$dnp`E 11.1 Examples
CX](^yU_ 11.2 Substrate Photoelectron Diffraction
E]G#"EV!Y 11.3 Adsorbate Photoelectron Diffraction
]ZJu 11.4 Fermi Surface Scans
:e9}k5kdk References
^`0^|u= 3;fuz Kk@b Appendix
3SbtN3 A.1 Table of Binding Energies
#"tHT<8 u A.2 Surface and Bulk Brillouin Zones of the Three Low-Index Faces of a Face—Centered Cubic(fcc)Crystal Face
MUo}Qi0K A.3 Compilation of Work Functions
o`B,Pt5vu References
34Q;& z\e Index