光电子谱技术是研究原子、分子、固体和表面电子
结构的一种非常有效的手段。本书全面
系统地介绍了
光电子谱技术的
原理和应用,并简明讨论了逆光发射、自旋极化光发射和
光电子衍射等现象。本书是一本非常实用的光电子谱技术的专著,内容几乎覆盖了光电子研究的所有领域。其特点是紧密联系实验,并利用理论详细解释实验结果,达到理论和应用的有机结合。书中还收集了大量的实际
材料的光电子谱分析,同时给出了大量的实验数据,以便于读者的查阅。总之,该书既是一本很有价值的参考书,又可作为初学者的入门教材。
~7+7{9g n^B9Mh@ 作者在该领域做出了杰出的贡献。在第3版中,作者介绍了大量最新研究成果,并对光电子谱技术很多方面给出了有深刻见解的讨论。
C-E~z{ c[J?`8 读者对象:适用于凝聚态
物理学、材料物理学和光电子学等专业的高年级本科生、研究生和相关专业的科研人员。
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nF>41 K -}Zck1 目录
0b6jGa 1. Introduction and Basic Principles
TwlX'iI_; 1.1 Historical Development
FlGU1%]m 1.2 The Electron Mean Free Path
6D|[3rXr 1.3 Photoelectron Spectroscopy and Inverse Photoelectron Spectroscopy
0`c|ZzY 1.4 Experimental Aspects
SQ8xfD* 1.5 Very High Resolution
vz5x{W 1.6 The Theory of Photoemission
m:B9~lbT+ 1.6.1 Core-Level Photoemission
F]e`-; 1.6.2 Valence-State Photoemission
7]W6\Z 1.6.3 Three-Step and One-Step Considerations
60,z! Vv 1.7 Deviations from the Simple Theory of Photoemission
2(LF @xb References
@W}cM -!;2?6R9{ 2. Core Levels and Final States
WoM;) Q 2.1 Core-Level Binding Energies in Atoms and Molecules
X3e&c 2.1.1 The Equivalent-Core Approximation
p 4_j>JPv5 2.1.2 Chemical Shifts
Ipro6
I 2.2 Core-Level Binding Energies in Solids
@<kY,ox@~ 2.2.1 The Born-Haber Cycle in Insulators
oCfO:7 2.2.2 Theory of Binding Energies
& "i4og< 2.2.3 Determination of Binding Energies and Chemical Shifts from Thermodynamic Data
-Zq\x' 2.3 Core Polarization
J,4,#2M8 2.4 Final-State Multiplets in Rare-Earth Valence Bands
=mR~\R(
I 2.5 Vibrational Side Bands
+t*V7nW 2.6 Core Levels of Adsorbed Molecules
U\*]cw 2.7 Quantitative Chemical Analysis from Core-Level Intensities
`eZzYe(N References
!Gob `# r DW(
/[jo\ 3. Charge-Excitation Final States: Satellites
Gyx4}pV 3.1 Copper Dihalides; 3d Transition Metal Compounds
(
jAC Lo 3.1.1 Characterization of a Satellite
4>^LEp 3.1.2 Analysis of Charge-Transfer Satellites
!/nXEjW? 3.1.3 Non-local Screening
37apOK4+ 3.2 The 6-eV Satellite in Nickel
"s-3226kj 3.2.1 Resonance Photoemission
LMKhtOZ? 3.2.2 Satellites in Other Metals
F m?j-' 3.3 The Gunnarsson-Sch6nhammer Theory
v[;R(pt? 3.4 Photoemission Signals and Narrow Bands in Metals
srPczVG* References
)<Fq}Q86 .RNY}bbk 4. Continuous Satellites and Plasmon Satellites: XPS Photoemission in Nearly Free Electron Systems
PRJ 4.1 Theory
~c,CngeL0 4.1.1 General
8Q%g<jX* 4.1.2 Core-Line Shape
>|X ) 4.1.3 Intrinsic Plasmons
vB74r]'F 4.1.4 Fxtrinsic FAectron Scattering: Plasmons and Background
|I[/Fl: 4.1.5 The Total Photoelectron Spectrum
yPrF2@#XZ/ 4.2 Experimental Results
6VUs:iO1j5 4.2.1 The Core Line Without Plasmons
\?v?%}x 4.2.2 Core-Level Spectra Including Plasmoas
r[?GO"ej5 4.2.3 Valence-Band Spectra of the Simple Metals
k5M5bH', 4.2.4 Simple Metals: A General Comment
H;nEU@>"Z 4.3 The Background Correction
*+OS;R1< References
M*!WXQlud @An} 5. Valence Orbitals in Simple Molecules and Insulating Solids
za%gD 5.1 UPS Spectra of Monatomic Gases
<%o9*)F 5.2 Photoelectron Spectra of Diatomic Molecules
3Fb9\2<H 5.3 Binding Energy of the H2 Molecule
Y5CDdn 5.4 Hydrides Isoelectronic with Noble Gases
]d67 HOyK Neon (Ne)
LZ34x: ,C Hydrogen Fluoride (HF)
_aeIK Water (H2O)
y'aK92pF: Ammonia (NH3)
M>E~eb/ Methane (CH4)
_01wRsm%2 5.5 Spectra of the Alkali HMides
=oBlUE 5.6 Transition Metal Dihalides
VV;%q3}: 5.7 Hydrocarbons
5U-SIG* 5.7.1 Guidelines for the Interpretation of Spectra from Free Molecules
vPz$+&{I 5.7.2 Linear Polymers
O1D|T"@ 5.8 Insulating Solids with Valence d Electrons
P_4E<"eK 5.8.1 The NiO Problem
JM1O7I 5.8.2 Mort Insulation
,ZghV1z 5.8.3 The Metal-Insulator Transition;the Ratio of the Correlation Energy and the Bandwidth;Doping
6hMKAk 5.8.4Band Structures of Transition Metal Compounds
Fc#Sn2p* 5.9 High—Temperature Superconductors
^T:L6: 5.9.1valence-Band Electronic Structure;Polycrystalline Samples
cYp/? \ 5.9.2 Dispersion Relations in High Temperature Superconductors;Single Crystals
:YQI1 q[6 5.9.3 The Superconducting Gap
lA%FS]vh 5.9.4 Symmetry of the Order Parameter in the High-Temperature SuDerconductors
UX+vU@Co[ 5.9.5 Core—Level Shifts
t~7OtPF 5.10 The Fermi Liquid and the Luttinger Liquid
0kSM$D_ 5.11 Adsorbed Molecules
Q^;:Kl.b 5.11.1 Outline
IyI0|&r2A 5.11.2 CO on Metal Surfaces
Bn9#F#F< References
O\CnKNk, 2eHVl.C5 6.Photoemission of Valence Electrons froill Metallic Solids in the OHe-Electron Approximation
"~=-Q#xO 6.1 Theory of Photoemission:A Summary of the Three-Step Model
GE`1j'^- 6.2 Discussion of the Photocurrent
3. @LAF 6.2.1 Kinematics of Internal Photoemission in a Polycrystalline Sample
y XKddD 6.2.2 Primary and Secondary Cones in the Photoemission from a Real Solid
EK=
y!> 6.2.3 Angle-Integrated and Angle-Resolved Data Collection
RC}m]!Uz 6.3 Photoemission from the Semi—infinite Crystal:The Inverse LEED Formalism
#i.,+Q 6.3.1 Band Structure Regime
"u]&~$ 6.3.2 XPS Regime
C6EGM/m8 6.3.3 Surface Emission
,{mv6?_ 6.3.4 One-Step Calculations
D Qz+t 6.4 Thermal Effects
Vpne-PW 6.5 Dipole Selection Rules for Direct Optical Transitions
"={* 0P References
PtYG%/s Y)DAR83 7.Band Structtire and Angular-Resolved Photoelectron Spectra
Pz34a@%" 7.1 Free-Electron Final—State Model
O/|))H?C 7.2 Methods Employing Calculated Band Structures
AT)b/ycC 7.3 Methods for the Absolute Determination of the Crystal Momentum
jz`3xFy *] 7.3.1 Triangulation or Energy Coincidence Method
I?St}Tl 7.3.2 Bragg Plane Method: Variation of External Emission Angle at Fixed Photon Frequency (Disappearance/Appearance Angle Method
k_{?{:X;y 7.3.3 Bragg Plane Method: Variation of Photon Energy at Fixed Emission Angle (Symmetry Method)
Y/6>OD 7.3.4 The Surface Emission Method and Electron Damping
lP*n%Pn) 7.3.5 The Very-Low-Energy Electron Diffraction Method
1
_Oc1RM 7.3.6 The Fermi Surface Method
%YK xdp 7.3.7 Intensities and Their Use in Band-Structure Determinations
Q?;Tc.O"/ 7.3.8 Summary
tu Y+n2 7.4 Experimental Band Structures
S.4+tf7+ 7.4.1 One- and Two-Dimensional Systems
hf]m'5pb 7.4.2 Three-Dimensional Solids: Metals and Semiconductors
[zBi*%5O 7..4.3UPS Band Structures and XPS Density of States
5@%.wb4 7.5 A Comment
T\n6^@.> References
r88De=* g0bYO!gCr 8.Surface States, Surface Effects
=/_u k{ 8.1 Theoretical Considerations
(M"rpG>L 8.2 Experimental Results on Surface States
qC{JsX`~ 8.3 Quantum-Well States
CvmIDRP* 8.4 Surface Core-Level Shifts
Gc"hU:m References
WB?HY?[r *2u~5Kc< 9.Inverse Photoelectron Spectroscopy
;:j1FOj 9.1 Surface States
zxx\jpBBk 9.2 Bulk Band Structures
|dqHpogh 9.3 Adsorbed Molecules
OtoM References
vjS=ZinN" ;<N:! $p 10. Spin-Polarized Photoelectron Spectroscopy
}rI:pp^KS 10.1 General Description
?!&%-R6* 10.2 Examples of Spin-Polarized Photoelectron Spectroscopy
%2T
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Rb 10.3 Magnetic Dichroism
|bz%SB References
#kASy 2t 6IG?t 11. Photoelectron Diffraction
6_4B! 11.1 Examples
BH1h2OEe# 11.2 Substrate Photoelectron Diffraction
,#UZp\zZ* 11.3 Adsorbate Photoelectron Diffraction
e~'lWJD 11.4 Fermi Surface Scans
iW^J>aKy References
E#!!tH`lgg l@Vv%w9H Appendix
;5bd<N A.1 Table of Binding Energies
?' .AeoE- A.2 Surface and Bulk Brillouin Zones of the Three Low-Index Faces of a Face—Centered Cubic(fcc)Crystal Face
R`cP%7K A.3 Compilation of Work Functions
@]vY[O!&; References
-1,0hmn=+ Index