光电子谱技术是研究原子、分子、固体和表面电子
结构的一种非常有效的手段。本书全面
系统地介绍了
光电子谱技术的
原理和应用,并简明讨论了逆光发射、自旋极化光发射和
光电子衍射等现象。本书是一本非常实用的光电子谱技术的专著,内容几乎覆盖了光电子研究的所有领域。其特点是紧密联系实验,并利用理论详细解释实验结果,达到理论和应用的有机结合。书中还收集了大量的实际
材料的光电子谱分析,同时给出了大量的实验数据,以便于读者的查阅。总之,该书既是一本很有价值的参考书,又可作为初学者的入门教材。
Xs)?PE[ ~tB9kLFG 作者在该领域做出了杰出的贡献。在第3版中,作者介绍了大量最新研究成果,并对光电子谱技术很多方面给出了有深刻见解的讨论。
n&E/{o( GJBMaT 读者对象:适用于凝聚态
物理学、材料物理学和光电子学等专业的高年级本科生、研究生和相关专业的科研人员。
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ZC&4uNUr / KKA/ 目录
deutY.7g 1. Introduction and Basic Principles
r6e!";w:U 1.1 Historical Development
q/3co86c 1.2 The Electron Mean Free Path
)GJlQ1x 1.3 Photoelectron Spectroscopy and Inverse Photoelectron Spectroscopy
5:l"* 1.4 Experimental Aspects
qjIcRue'" 1.5 Very High Resolution
>V@,K z1 1.6 The Theory of Photoemission
^I!gteU; 1.6.1 Core-Level Photoemission
83:qIfF 1.6.2 Valence-State Photoemission
&-ZRS/_d> 1.6.3 Three-Step and One-Step Considerations
5K|s]Y; 1.7 Deviations from the Simple Theory of Photoemission
jHc/ EZB References
)H1chNI) Bzr}+J 2. Core Levels and Final States
bt?)ryu 2.1 Core-Level Binding Energies in Atoms and Molecules
,+RoJwi m 2.1.1 The Equivalent-Core Approximation
/Pa<I^-# 2.1.2 Chemical Shifts
%l)~C%T 2.2 Core-Level Binding Energies in Solids
$dHD 2.2.1 The Born-Haber Cycle in Insulators
8?k.4{? 2.2.2 Theory of Binding Energies
LP}YHW/ 2.2.3 Determination of Binding Energies and Chemical Shifts from Thermodynamic Data
r7N%onx 2.3 Core Polarization
7>|p_o`e 2.4 Final-State Multiplets in Rare-Earth Valence Bands
o`[X _ 2.5 Vibrational Side Bands
+4Lj}8, 2.6 Core Levels of Adsorbed Molecules
,5Tw5<S 2.7 Quantitative Chemical Analysis from Core-Level Intensities
Jf8AKj3 References
.(zZTyZr ak;S Ie 3. Charge-Excitation Final States: Satellites
dLTA21b# 3.1 Copper Dihalides; 3d Transition Metal Compounds
%q,^A+= 3.1.1 Characterization of a Satellite
K?aUIkVs 3.1.2 Analysis of Charge-Transfer Satellites
=;A~$[ g 3.1.3 Non-local Screening
,=p.Cx'PR 3.2 The 6-eV Satellite in Nickel
;:pd/\< 3.2.1 Resonance Photoemission
Q Ph6
p3bg 3.2.2 Satellites in Other Metals
<x2 F5$@ 3.3 The Gunnarsson-Sch6nhammer Theory
Mt`XHXTp 3.4 Photoemission Signals and Narrow Bands in Metals
j\8'P9~% References
s
*1%I$=@ Sf0[^"7 4. Continuous Satellites and Plasmon Satellites: XPS Photoemission in Nearly Free Electron Systems
},LW@Z} 4.1 Theory
yw)Ztg) 4.1.1 General
Gk5SG_o 4.1.2 Core-Line Shape
\M`fkR,,' 4.1.3 Intrinsic Plasmons
h8_~ OX 4.1.4 Fxtrinsic FAectron Scattering: Plasmons and Background
CVFsp>+ 4.1.5 The Total Photoelectron Spectrum
&vp0zYd+v 4.2 Experimental Results
<=,KP) 4.2.1 The Core Line Without Plasmons
?V&[U 4.2.2 Core-Level Spectra Including Plasmoas
oxPb; % 4.2.3 Valence-Band Spectra of the Simple Metals
L"6@3 4.2.4 Simple Metals: A General Comment
?k:i3$ 4.3 The Background Correction
cIgicp}U References
Eqva]
4 ZWJFd(6 5. Valence Orbitals in Simple Molecules and Insulating Solids
Aq{m42EAj 5.1 UPS Spectra of Monatomic Gases
Uq6..<# 5.2 Photoelectron Spectra of Diatomic Molecules
Yg#)@L 5.3 Binding Energy of the H2 Molecule
k|7XC@i]% 5.4 Hydrides Isoelectronic with Noble Gases
rkl/5z?? Neon (Ne)
J)n g,i Hydrogen Fluoride (HF)
\(LHcvbb Water (H2O)
#|8!0]n' Ammonia (NH3)
@]HV:7<q Methane (CH4)
$sO}l 5.5 Spectra of the Alkali HMides
D] 2+<;>`> 5.6 Transition Metal Dihalides
3P p*ID 5.7 Hydrocarbons
qD#-q vn 5.7.1 Guidelines for the Interpretation of Spectra from Free Molecules
9bXU!l[ 5.7.2 Linear Polymers
r/L3j0 5.8 Insulating Solids with Valence d Electrons
3<msiCP 5.8.1 The NiO Problem
W.n@ 5.8.2 Mort Insulation
(s{%XB:K 5.8.3 The Metal-Insulator Transition;the Ratio of the Correlation Energy and the Bandwidth;Doping
Q;5'I3w 5.8.4Band Structures of Transition Metal Compounds
hv
.Mf.m 5.9 High—Temperature Superconductors
tQJ@//C\z 5.9.1valence-Band Electronic Structure;Polycrystalline Samples
N
&p=4 5.9.2 Dispersion Relations in High Temperature Superconductors;Single Crystals
qg6Hk:^r 5.9.3 The Superconducting Gap
%_SE$>v^ 5.9.4 Symmetry of the Order Parameter in the High-Temperature SuDerconductors
Ed*`d> 5.9.5 Core—Level Shifts
{Rw~G&vQ 5.10 The Fermi Liquid and the Luttinger Liquid
7qXgHrr0|U 5.11 Adsorbed Molecules
T:.J9 5.11.1 Outline
e@^}y4
C 5.11.2 CO on Metal Surfaces
dt3Vy*zL References
r?/>t1Z o
ohf)) 6.Photoemission of Valence Electrons froill Metallic Solids in the OHe-Electron Approximation
^Z:x poz, 6.1 Theory of Photoemission:A Summary of the Three-Step Model
a9jY^E'|n 6.2 Discussion of the Photocurrent
E4y"$U%. 6.2.1 Kinematics of Internal Photoemission in a Polycrystalline Sample
n7<<}wcV 6.2.2 Primary and Secondary Cones in the Photoemission from a Real Solid
!b _<_Y{l 6.2.3 Angle-Integrated and Angle-Resolved Data Collection
KS(T%mk\ 6.3 Photoemission from the Semi—infinite Crystal:The Inverse LEED Formalism
x5`q)!<& 6.3.1 Band Structure Regime
"v*RY "5# 6.3.2 XPS Regime
"l +Jx|h\ 6.3.3 Surface Emission
6u:5]e8 6.3.4 One-Step Calculations
29Q5s$YD@ 6.4 Thermal Effects
KI>7h.t 6.5 Dipole Selection Rules for Direct Optical Transitions
PL+fLCk,I References
J;T_9 c@nl;u)n 7.Band Structtire and Angular-Resolved Photoelectron Spectra
)If[pw@j 7.1 Free-Electron Final—State Model
s:]rL&| 7.2 Methods Employing Calculated Band Structures
@fE^w^K7 7.3 Methods for the Absolute Determination of the Crystal Momentum
(c[h,>`@: 7.3.1 Triangulation or Energy Coincidence Method
/CA)R26G 7.3.2 Bragg Plane Method: Variation of External Emission Angle at Fixed Photon Frequency (Disappearance/Appearance Angle Method
3UN Jj&-` 7.3.3 Bragg Plane Method: Variation of Photon Energy at Fixed Emission Angle (Symmetry Method)
>2g CM 7.3.4 The Surface Emission Method and Electron Damping
0|^x[dh 7.3.5 The Very-Low-Energy Electron Diffraction Method
Fsq S) 7.3.6 The Fermi Surface Method
Yaa
M-o 7.3.7 Intensities and Their Use in Band-Structure Determinations
([9h.M6v 7.3.8 Summary
caj) 7.4 Experimental Band Structures
RXWjFv~/ 7.4.1 One- and Two-Dimensional Systems
]7u8m[@ 7.4.2 Three-Dimensional Solids: Metals and Semiconductors
z~VA#8> 7..4.3UPS Band Structures and XPS Density of States
v\MH;DW^Z 7.5 A Comment
|[{;*wtv References
,<vrDHR
40c#zCE 8.Surface States, Surface Effects
`jZX(H 8.1 Theoretical Considerations
'Vrev8D 8.2 Experimental Results on Surface States
lMm-K%(2 8.3 Quantum-Well States
}zobIfIF 8.4 Surface Core-Level Shifts
N0qC/da1 References
6=@n
b3D% I Mv^ 9T: 9.Inverse Photoelectron Spectroscopy
s?6 7@\ 9.1 Surface States
)>Lsj1qk 9.2 Bulk Band Structures
D1j7iv 9.3 Adsorbed Molecules
OUdeQO? References
O?2<rbx c'|MC[^A 10. Spin-Polarized Photoelectron Spectroscopy
cUm9s>^)/ 10.1 General Description
%&]}P;& 10.2 Examples of Spin-Polarized Photoelectron Spectroscopy
@"/}Al 10.3 Magnetic Dichroism
Q./lX: References
-E500F*b cdfll+ 11. Photoelectron Diffraction
kCC9U_dj, 11.1 Examples
kCwTv:) 11.2 Substrate Photoelectron Diffraction
aEk*-v#{ 11.3 Adsorbate Photoelectron Diffraction
6m.Ku13; 11.4 Fermi Surface Scans
z1FbW&V References
I|j tpv} (O-)uC Appendix
z^Jl4V A.1 Table of Binding Energies
PPqTmx5S A.2 Surface and Bulk Brillouin Zones of the Three Low-Index Faces of a Face—Centered Cubic(fcc)Crystal Face
&53#`WgJ A.3 Compilation of Work Functions
Fm;)7.%
> References
9V],X=y~ Index