光电子谱技术是研究原子、分子、固体和表面电子
结构的一种非常有效的手段。本书全面
系统地介绍了
光电子谱技术的
原理和应用,并简明讨论了逆光发射、自旋极化光发射和
光电子衍射等现象。本书是一本非常实用的光电子谱技术的专著,内容几乎覆盖了光电子研究的所有领域。其特点是紧密联系实验,并利用理论详细解释实验结果,达到理论和应用的有机结合。书中还收集了大量的实际
材料的光电子谱分析,同时给出了大量的实验数据,以便于读者的查阅。总之,该书既是一本很有价值的参考书,又可作为初学者的入门教材。
O>UR\l|+:2 8dP^zjPj 作者在该领域做出了杰出的贡献。在第3版中,作者介绍了大量最新研究成果,并对光电子谱技术很多方面给出了有深刻见解的讨论。
>=wlS\:" KATt9ox@ 读者对象:适用于凝聚态
物理学、材料物理学和光电子学等专业的高年级本科生、研究生和相关专业的科研人员。
Nb-;D)W;B ^MuO;<<,.
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c{zQX0 K^EW*6vB8O 目录
P/4]x@{ih 1. Introduction and Basic Principles
5Osx__6 $t 1.1 Historical Development
]JbGP{UiN 1.2 The Electron Mean Free Path
o@vo,JU 1.3 Photoelectron Spectroscopy and Inverse Photoelectron Spectroscopy
2]hQ56Yv3 1.4 Experimental Aspects
8e x{N3 1.5 Very High Resolution
6Wl+5
a6V 1.6 The Theory of Photoemission
`|[Q]+Mx 1.6.1 Core-Level Photoemission
*zJ}=%)f 1.6.2 Valence-State Photoemission
nKT\ /}d 1.6.3 Three-Step and One-Step Considerations
Ab/gY$l 1.7 Deviations from the Simple Theory of Photoemission
|X0h-kX4 References
>2TDYB|; 2/3,%5j_ 2. Core Levels and Final States
,,OO2EgZ` 2.1 Core-Level Binding Energies in Atoms and Molecules
O)n"a\LD 2.1.1 The Equivalent-Core Approximation
CtfI&rb[ 2.1.2 Chemical Shifts
%N04k8z 2.2 Core-Level Binding Energies in Solids
|\Nu+w 2.2.1 The Born-Haber Cycle in Insulators
h${+{1](6 2.2.2 Theory of Binding Energies
D:4Iex9$F" 2.2.3 Determination of Binding Energies and Chemical Shifts from Thermodynamic Data
R_`i=>Z- 2.3 Core Polarization
To.CY^M 2.4 Final-State Multiplets in Rare-Earth Valence Bands
B|zJrz0q3 2.5 Vibrational Side Bands
(
$A0b 2.6 Core Levels of Adsorbed Molecules
1:(qoA: 2.7 Quantitative Chemical Analysis from Core-Level Intensities
!`JaYUL[e References
]yy10Pk[! KEEHb2q 3. Charge-Excitation Final States: Satellites
Dyyf%'\M 3.1 Copper Dihalides; 3d Transition Metal Compounds
],V_"\ATD 3.1.1 Characterization of a Satellite
&'Pwz 3.1.2 Analysis of Charge-Transfer Satellites
*]:gEO 3.1.3 Non-local Screening
9!&fak_ 3.2 The 6-eV Satellite in Nickel
ux:czZqy 3.2.1 Resonance Photoemission
wylbs@ 3.2.2 Satellites in Other Metals
kZ~ 0fw- 3.3 The Gunnarsson-Sch6nhammer Theory
d0vn/k2I 3.4 Photoemission Signals and Narrow Bands in Metals
z|E/pm$^ References
L|A}A[ P )RG@D\t , 4. Continuous Satellites and Plasmon Satellites: XPS Photoemission in Nearly Free Electron Systems
lV<2+Is 4.1 Theory
e)"]H* 4.1.1 General
]?tC+UKb 4.1.2 Core-Line Shape
fyaiRn9/ 4.1.3 Intrinsic Plasmons
9$U@h7|Q` 4.1.4 Fxtrinsic FAectron Scattering: Plasmons and Background
%&w 8E[ 4.1.5 The Total Photoelectron Spectrum
LX;w~fRr. 4.2 Experimental Results
]zK'aod 4.2.1 The Core Line Without Plasmons
Y>W$n9d&G2 4.2.2 Core-Level Spectra Including Plasmoas
lV924mh 4.2.3 Valence-Band Spectra of the Simple Metals
;aXu 4.2.4 Simple Metals: A General Comment
2^RWGCEv 4.3 The Background Correction
Vz_ac
vfk^ References
^C$Oht,cU t+y$i@R: 5. Valence Orbitals in Simple Molecules and Insulating Solids
4j+FDc` 5.1 UPS Spectra of Monatomic Gases
|[qq
$ 5.2 Photoelectron Spectra of Diatomic Molecules
=Y!x 5.3 Binding Energy of the H2 Molecule
j=c=Pe"?u 5.4 Hydrides Isoelectronic with Noble Gases
,t?c=u\5 Neon (Ne)
[Ume^ Hydrogen Fluoride (HF)
17kh6(X Water (H2O)
2w"Xv,*.'i Ammonia (NH3)
3>vSKh1z Methane (CH4)
IY_u|7d 5.5 Spectra of the Alkali HMides
yR}PC/> 5.6 Transition Metal Dihalides
Q5Yy
\M 5.7 Hydrocarbons
[=/Yo1:v 5.7.1 Guidelines for the Interpretation of Spectra from Free Molecules
bT93R8yp 5.7.2 Linear Polymers
Z8mSm[w 5.8 Insulating Solids with Valence d Electrons
^<u9I5? 5.8.1 The NiO Problem
"$P|!k45( 5.8.2 Mort Insulation
#WE"nh9f|z 5.8.3 The Metal-Insulator Transition;the Ratio of the Correlation Energy and the Bandwidth;Doping
Z!#n55| 5.8.4Band Structures of Transition Metal Compounds
j<,Ho4v}_ 5.9 High—Temperature Superconductors
B"; >zF 5.9.1valence-Band Electronic Structure;Polycrystalline Samples
hv.33l 5.9.2 Dispersion Relations in High Temperature Superconductors;Single Crystals
MC\rx=cR\ 5.9.3 The Superconducting Gap
@bfW-\ I 5.9.4 Symmetry of the Order Parameter in the High-Temperature SuDerconductors
,EsPm'`?A/ 5.9.5 Core—Level Shifts
[te9ui%JS 5.10 The Fermi Liquid and the Luttinger Liquid
\Dn47V{7- 5.11 Adsorbed Molecules
KkD.n#A 5.11.1 Outline
x&^>|'H 5.11.2 CO on Metal Surfaces
oY
NIJXln References
6>L) vH[G#A~4 6.Photoemission of Valence Electrons froill Metallic Solids in the OHe-Electron Approximation
Uw`YlUT\ 6.1 Theory of Photoemission:A Summary of the Three-Step Model
c
qWX*&2_ 6.2 Discussion of the Photocurrent
,?k0~fuG6 6.2.1 Kinematics of Internal Photoemission in a Polycrystalline Sample
cpY'::5.% 6.2.2 Primary and Secondary Cones in the Photoemission from a Real Solid
<xn96|$ 6.2.3 Angle-Integrated and Angle-Resolved Data Collection
;pH&YBY 6.3 Photoemission from the Semi—infinite Crystal:The Inverse LEED Formalism
$~^Y4 }
m 6.3.1 Band Structure Regime
TK! D=M 6.3.2 XPS Regime
<q}w, XU 6.3.3 Surface Emission
_R/^P>Q? 6.3.4 One-Step Calculations
Nd;)V 6.4 Thermal Effects
27"M]17) 6.5 Dipole Selection Rules for Direct Optical Transitions
KzgW+6*G References
An.Qi =Cv sLHUQ(S! 7.Band Structtire and Angular-Resolved Photoelectron Spectra
9>QGsf.3 7.1 Free-Electron Final—State Model
PQ0l <]Y 7.2 Methods Employing Calculated Band Structures
Jm#mC 7.3 Methods for the Absolute Determination of the Crystal Momentum
]'"aVGqa. 7.3.1 Triangulation or Energy Coincidence Method
j:Y1 7.3.2 Bragg Plane Method: Variation of External Emission Angle at Fixed Photon Frequency (Disappearance/Appearance Angle Method
'nx";[6( 7.3.3 Bragg Plane Method: Variation of Photon Energy at Fixed Emission Angle (Symmetry Method)
n "J+?~9 7.3.4 The Surface Emission Method and Electron Damping
^Fop/\E 7.3.5 The Very-Low-Energy Electron Diffraction Method
&gv{LJd5b 7.3.6 The Fermi Surface Method
v,eTDgw 7.3.7 Intensities and Their Use in Band-Structure Determinations
jIvSjlm I 7.3.8 Summary
{p90 7.4 Experimental Band Structures
sJ3O ] 7.4.1 One- and Two-Dimensional Systems
9y$"[d27;+ 7.4.2 Three-Dimensional Solids: Metals and Semiconductors
M9PzA'}4W6 7..4.3UPS Band Structures and XPS Density of States
)8,) &F 7.5 A Comment
+t8{aaV References
n1E^8[~' ~#]$YoQ&O 8.Surface States, Surface Effects
VX'cFqrK3 8.1 Theoretical Considerations
B*
hW 8.2 Experimental Results on Surface States
,ve$bSp 8.3 Quantum-Well States
Ho^rYz 8.4 Surface Core-Level Shifts
.[Hv/?L References
$~G=Hcl9 f3E%0cg 9.Inverse Photoelectron Spectroscopy
12olVTuw 9.1 Surface States
[t{ed)J 9.2 Bulk Band Structures
Q>QES-.l 9.3 Adsorbed Molecules
:~PzTUz References
Vi:<W0: w(6(Fze 10. Spin-Polarized Photoelectron Spectroscopy
Cju%CE3a 10.1 General Description
%=PGvu 10.2 Examples of Spin-Polarized Photoelectron Spectroscopy
=7l'3z8 10.3 Magnetic Dichroism
_oU}>5 References
ajJ+Jn\ s9 \HjK*+ 11. Photoelectron Diffraction
m Bc2x8g) 11.1 Examples
:}n\
r/i 11.2 Substrate Photoelectron Diffraction
PKK18E}{%^ 11.3 Adsorbate Photoelectron Diffraction
DtRu&>o_6D 11.4 Fermi Surface Scans
}b$W+/M\ References
}$wWX}@ +`p@md2L1 Appendix
(Z)F6sZ`8 A.1 Table of Binding Energies
F?jFFwim A.2 Surface and Bulk Brillouin Zones of the Three Low-Index Faces of a Face—Centered Cubic(fcc)Crystal Face
/t$J<bU A.3 Compilation of Work Functions
49Y_ze6L} References
P)k!#* Index