光电子谱技术是研究原子、分子、固体和表面电子
结构的一种非常有效的手段。本书全面
系统地介绍了
光电子谱技术的
原理和应用,并简明讨论了逆光发射、自旋极化光发射和
光电子衍射等现象。本书是一本非常实用的光电子谱技术的专著,内容几乎覆盖了光电子研究的所有领域。其特点是紧密联系实验,并利用理论详细解释实验结果,达到理论和应用的有机结合。书中还收集了大量的实际
材料的光电子谱分析,同时给出了大量的实验数据,以便于读者的查阅。总之,该书既是一本很有价值的参考书,又可作为初学者的入门教材。
x_c7R;C ;x:rZV/ 作者在该领域做出了杰出的贡献。在第3版中,作者介绍了大量最新研究成果,并对光电子谱技术很多方面给出了有深刻见解的讨论。
~v'3"k6 $<^u^q37u 读者对象:适用于凝聚态
物理学、材料物理学和光电子学等专业的高年级本科生、研究生和相关专业的科研人员。
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8E4mA5@ 81hbk(( 目录
^2$ lJ 1. Introduction and Basic Principles
3/b;7\M 1.1 Historical Development
=xNv\e 1.2 The Electron Mean Free Path
^S)cjH`P 1.3 Photoelectron Spectroscopy and Inverse Photoelectron Spectroscopy
: C b&v07 1.4 Experimental Aspects
I
j$lDJS 1.5 Very High Resolution
1~l
I8 1.6 The Theory of Photoemission
5*E#*H 1.6.1 Core-Level Photoemission
c\ia6[3sX 1.6.2 Valence-State Photoemission
<JV"@H= 1.6.3 Three-Step and One-Step Considerations
rQEyD 1.7 Deviations from the Simple Theory of Photoemission
RPIyO References
C=s1R;"H aB]m*~ 2. Core Levels and Final States
$b<6y/" 2.1 Core-Level Binding Energies in Atoms and Molecules
k51Eyy50( 2.1.1 The Equivalent-Core Approximation
<`jLY)sw 2.1.2 Chemical Shifts
u$D*tqxG 2.2 Core-Level Binding Energies in Solids
0vVV%,v 2.2.1 The Born-Haber Cycle in Insulators
QT9n,lX 2.2.2 Theory of Binding Energies
Dk+&X-]6x5 2.2.3 Determination of Binding Energies and Chemical Shifts from Thermodynamic Data
kl"+YF5/ 2.3 Core Polarization
Qb!PRCHQ 2.4 Final-State Multiplets in Rare-Earth Valence Bands
!q-f9E4` 2.5 Vibrational Side Bands
gqR)IVk>% 2.6 Core Levels of Adsorbed Molecules
2_ :n 2.7 Quantitative Chemical Analysis from Core-Level Intensities
eeHP&1= 7 References
R-Z~V [!
'op0 3. Charge-Excitation Final States: Satellites
.AYj'Y 3.1 Copper Dihalides; 3d Transition Metal Compounds
qim
'dp: 3.1.1 Characterization of a Satellite
=1P6Vk 3.1.2 Analysis of Charge-Transfer Satellites
6Z`R#d #I 3.1.3 Non-local Screening
kPQtQh]y% 3.2 The 6-eV Satellite in Nickel
$2<d<Um~z 3.2.1 Resonance Photoemission
BW"&6t#kA 3.2.2 Satellites in Other Metals
}hYZ"
A~ 3.3 The Gunnarsson-Sch6nhammer Theory
<BO)E( 3.4 Photoemission Signals and Narrow Bands in Metals
ifo7%XPcg References
gtYAHi n39t}`WIl 4. Continuous Satellites and Plasmon Satellites: XPS Photoemission in Nearly Free Electron Systems
ltkI}h,e 4.1 Theory
;SwMu@tg 4.1.1 General
U|HB=BP 4.1.2 Core-Line Shape
wZ4tCZA 4.1.3 Intrinsic Plasmons
]`bQW? 4.1.4 Fxtrinsic FAectron Scattering: Plasmons and Background
GZ{]0$9I' 4.1.5 The Total Photoelectron Spectrum
oQv3GpO 4.2 Experimental Results
oG7q_4+& 4.2.1 The Core Line Without Plasmons
yQ3OL# 4.2.2 Core-Level Spectra Including Plasmoas
+kq'+ Y7 4.2.3 Valence-Band Spectra of the Simple Metals
.))v0 4.2.4 Simple Metals: A General Comment
/XudV2P-CA 4.3 The Background Correction
t+?P^Ok References
LTJc,3\,
t8+_/BXv 5. Valence Orbitals in Simple Molecules and Insulating Solids
,-+"^> 5.1 UPS Spectra of Monatomic Gases
OEPa|rb 5.2 Photoelectron Spectra of Diatomic Molecules
`xiCm': 5.3 Binding Energy of the H2 Molecule
6{,HiY 5.4 Hydrides Isoelectronic with Noble Gases
kQaSbpNmH Neon (Ne)
Fkf97Oi Hydrogen Fluoride (HF)
m~lpyAw Water (H2O)
w_ {,<[# Ammonia (NH3)
`z0{S! Methane (CH4)
#q3l!3\mW 5.5 Spectra of the Alkali HMides
`:O\dN>ON 5.6 Transition Metal Dihalides
P ]i
=r] i 5.7 Hydrocarbons
_U{([M>; 5.7.1 Guidelines for the Interpretation of Spectra from Free Molecules
Gn)y>
AN 5.7.2 Linear Polymers
bS
>0DU 5.8 Insulating Solids with Valence d Electrons
F`nb21{0y& 5.8.1 The NiO Problem
Qm8)4?FZ 5.8.2 Mort Insulation
z4@k$
L8 5.8.3 The Metal-Insulator Transition;the Ratio of the Correlation Energy and the Bandwidth;Doping
^`SA'F, 5.8.4Band Structures of Transition Metal Compounds
Y~)T 5.9 High—Temperature Superconductors
>xA),^ YT 5.9.1valence-Band Electronic Structure;Polycrystalline Samples
=SD\Q!fA 5.9.2 Dispersion Relations in High Temperature Superconductors;Single Crystals
>/<:Q & 5.9.3 The Superconducting Gap
^v9|%^ug 5.9.4 Symmetry of the Order Parameter in the High-Temperature SuDerconductors
]O{u tm 5.9.5 Core—Level Shifts
W>M~Sk$v 5.10 The Fermi Liquid and the Luttinger Liquid
g(O;{Q_ 5.11 Adsorbed Molecules
g\GdkiIj 5.11.1 Outline
~|wos-nM 5.11.2 CO on Metal Surfaces
hF3&i=;. References
s cdtWA +Z!;P
Z6 6.Photoemission of Valence Electrons froill Metallic Solids in the OHe-Electron Approximation
_ nP;Fx 6.1 Theory of Photoemission:A Summary of the Three-Step Model
M+wt__vHf 6.2 Discussion of the Photocurrent
>QHo@Zqj( 6.2.1 Kinematics of Internal Photoemission in a Polycrystalline Sample
w62=06`@ 6.2.2 Primary and Secondary Cones in the Photoemission from a Real Solid
>x3ug]Bu 6.2.3 Angle-Integrated and Angle-Resolved Data Collection
)'Wb&A' 6.3 Photoemission from the Semi—infinite Crystal:The Inverse LEED Formalism
W9t"aZor 6.3.1 Band Structure Regime
j<pw\k{i 6.3.2 XPS Regime
.[DthEF 6.3.3 Surface Emission
i`)!X:j 6.3.4 One-Step Calculations
aFY_:.o2k` 6.4 Thermal Effects
dSIH9D 6.5 Dipole Selection Rules for Direct Optical Transitions
<B /5J:o< References
,jy*1Hjd Ip}Vb6} 7.Band Structtire and Angular-Resolved Photoelectron Spectra
kW6%32 7.1 Free-Electron Final—State Model
Sx]
T/xq 7.2 Methods Employing Calculated Band Structures
Lc<eRVNd, 7.3 Methods for the Absolute Determination of the Crystal Momentum
+Ra3bj l 7.3.1 Triangulation or Energy Coincidence Method
1Q}mf !Y 7.3.2 Bragg Plane Method: Variation of External Emission Angle at Fixed Photon Frequency (Disappearance/Appearance Angle Method
~un%4]U 7.3.3 Bragg Plane Method: Variation of Photon Energy at Fixed Emission Angle (Symmetry Method)
J
NC 7.3.4 The Surface Emission Method and Electron Damping
:f'&z47 7.3.5 The Very-Low-Energy Electron Diffraction Method
&"uV~AM 7.3.6 The Fermi Surface Method
\g-j9|0 7.3.7 Intensities and Their Use in Band-Structure Determinations
!c<w SQ, 7.3.8 Summary
GR'Ti*Qi 7.4 Experimental Band Structures
2aw&F Z? 7.4.1 One- and Two-Dimensional Systems
dMl+ko 7.4.2 Three-Dimensional Solids: Metals and Semiconductors
tJ&5tNl 7..4.3UPS Band Structures and XPS Density of States
2
Tvvq(?T 7.5 A Comment
*! :QdWLq References
%-;bu| tn/T6C^) 8.Surface States, Surface Effects
>s*Drf X6 8.1 Theoretical Considerations
=OTm2:j#yQ 8.2 Experimental Results on Surface States
}xn_6 8.3 Quantum-Well States
y[0`hSQ)~ 8.4 Surface Core-Level Shifts
lm'Zy"~:: References
ED3?rXsSR Appendix
"/%89 HMD A.1 Table of Binding Energies
;\b@)E} A.2 Surface and Bulk Brillouin Zones of the Three Low-Index Faces of a Face—Centered Cubic(fcc)Crystal Face
*FgJ|y6gk A.3 Compilation of Work Functions
XYbyOM VI References
M^SuV Index