光电子谱技术是研究原子、分子、固体和表面电子
结构的一种非常有效的手段。本书全面
系统地介绍了
光电子谱技术的
原理和应用,并简明讨论了逆光发射、自旋极化光发射和
光电子衍射等现象。本书是一本非常实用的光电子谱技术的专著,内容几乎覆盖了光电子研究的所有领域。其特点是紧密联系实验,并利用理论详细解释实验结果,达到理论和应用的有机结合。书中还收集了大量的实际
材料的光电子谱分析,同时给出了大量的实验数据,以便于读者的查阅。总之,该书既是一本很有价值的参考书,又可作为初学者的入门教材。
&9Xn:<"`) / MV2#P@ 作者在该领域做出了杰出的贡献。在第3版中,作者介绍了大量最新研究成果,并对光电子谱技术很多方面给出了有深刻见解的讨论。
L#Rj~&U prO ~g 读者对象:适用于凝聚态
物理学、材料物理学和光电子学等专业的高年级本科生、研究生和相关专业的科研人员。
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:?f^D,w_B y?ypRCgO.u 目录
\<Di|X1 1. Introduction and Basic Principles
/5"RedP< 1.1 Historical Development
|ohCA&k%; 1.2 The Electron Mean Free Path
!T
RU 1.3 Photoelectron Spectroscopy and Inverse Photoelectron Spectroscopy
'l6SL-
< 1.4 Experimental Aspects
m)e~HP7M 1.5 Very High Resolution
uQO\vRh0 1.6 The Theory of Photoemission
CC|=$(PgT 1.6.1 Core-Level Photoemission
8&c:73=?X 1.6.2 Valence-State Photoemission
$n_ax\15 1.6.3 Three-Step and One-Step Considerations
Uj twOv|pF 1.7 Deviations from the Simple Theory of Photoemission
]oizBa@?G References
]!v\whZ> dlCmSCp% 2. Core Levels and Final States
7[It 2.1 Core-Level Binding Energies in Atoms and Molecules
`[F[0fY- 2.1.1 The Equivalent-Core Approximation
z4wG]]Kh* 2.1.2 Chemical Shifts
7;$[s6$ 2.2 Core-Level Binding Energies in Solids
- sL4tMP 2.2.1 The Born-Haber Cycle in Insulators
(Z?g^kjq) 2.2.2 Theory of Binding Energies
Yk=2ld;; 2.2.3 Determination of Binding Energies and Chemical Shifts from Thermodynamic Data
~vB dq Yj 2.3 Core Polarization
iG+=whvL 2.4 Final-State Multiplets in Rare-Earth Valence Bands
2}U:6w 2.5 Vibrational Side Bands
L^e%oQ>s 2.6 Core Levels of Adsorbed Molecules
!]l;n
Fd 2.7 Quantitative Chemical Analysis from Core-Level Intensities
Q&8epO |J References
7O<K?;I Dn@Sjsj> 3. Charge-Excitation Final States: Satellites
|C}= 1 3.1 Copper Dihalides; 3d Transition Metal Compounds
npMPjknl 3.1.1 Characterization of a Satellite
x/uC)xm 3.1.2 Analysis of Charge-Transfer Satellites
/kNSB; 3.1.3 Non-local Screening
`Tc"a_p9t 3.2 The 6-eV Satellite in Nickel
9"f 3.2.1 Resonance Photoemission
.wf$]oQQ 3.2.2 Satellites in Other Metals
]BaK8mPl 3.3 The Gunnarsson-Sch6nhammer Theory
Hgbrlh 3.4 Photoemission Signals and Narrow Bands in Metals
, d7o/8u References
T~)R,OA7m {9XQ~t"m^ 4. Continuous Satellites and Plasmon Satellites: XPS Photoemission in Nearly Free Electron Systems
G!E1N(%o 4.1 Theory
y;=/S?L.: 4.1.1 General
Y3bZ&G) 4.1.2 Core-Line Shape
%OJq( } 4.1.3 Intrinsic Plasmons
HiSNEp$-4$ 4.1.4 Fxtrinsic FAectron Scattering: Plasmons and Background
hFMT@Gy 4.1.5 The Total Photoelectron Spectrum
E{]PfUfFY 4.2 Experimental Results
Jp-6]uW 4.2.1 The Core Line Without Plasmons
BQL](Y" 4.2.2 Core-Level Spectra Including Plasmoas
%s ">: 4.2.3 Valence-Band Spectra of the Simple Metals
}TRVCF1 4.2.4 Simple Metals: A General Comment
?6 //'bO:% 4.3 The Background Correction
z9JZV`dNgz References
S^_F0</U, bFsJqA.A 5. Valence Orbitals in Simple Molecules and Insulating Solids
>j)y7DSE 5.1 UPS Spectra of Monatomic Gases
d'[] 5.2 Photoelectron Spectra of Diatomic Molecules
q+W*?a) 5.3 Binding Energy of the H2 Molecule
lf}%^od~6 5.4 Hydrides Isoelectronic with Noble Gases
*Ke\Yb Neon (Ne)
$PFE>=nM Hydrogen Fluoride (HF)
Eg4_kp0Lq Water (H2O)
{ZKXT8' Ammonia (NH3)
Xd5uF/w Methane (CH4)
C=&;4In 5.5 Spectra of the Alkali HMides
PGhYkj2 5.6 Transition Metal Dihalides
`Hd~H 5.7 Hydrocarbons
l09DH+ 5.7.1 Guidelines for the Interpretation of Spectra from Free Molecules
YcN &\( 5.7.2 Linear Polymers
(w-@b70E 5.8 Insulating Solids with Valence d Electrons
);d"gv(]D 5.8.1 The NiO Problem
0,j!* 5.8.2 Mort Insulation
s^HI%mdf 5.8.3 The Metal-Insulator Transition;the Ratio of the Correlation Energy and the Bandwidth;Doping
Y7<(_p7 5.8.4Band Structures of Transition Metal Compounds
DhN<e7c` 5.9 High—Temperature Superconductors
{9-n3j} 5.9.1valence-Band Electronic Structure;Polycrystalline Samples
liPaT 5.9.2 Dispersion Relations in High Temperature Superconductors;Single Crystals
Y'76! Y 5.9.3 The Superconducting Gap
#7=- zda5 5.9.4 Symmetry of the Order Parameter in the High-Temperature SuDerconductors
3`Gb;D 5.9.5 Core—Level Shifts
DVjwY_nG7 5.10 The Fermi Liquid and the Luttinger Liquid
2#R8}\ 5.11 Adsorbed Molecules
3ICM H
5.11.1 Outline
^CW{`eBwk 5.11.2 CO on Metal Surfaces
23/;W| References
M=Y['wx Kon|TeC>d 6.Photoemission of Valence Electrons froill Metallic Solids in the OHe-Electron Approximation
6/.cS4 6.1 Theory of Photoemission:A Summary of the Three-Step Model
]MnQ3bWq"j 6.2 Discussion of the Photocurrent
h_15 " rd 6.2.1 Kinematics of Internal Photoemission in a Polycrystalline Sample
Sh\Jm*5 6.2.2 Primary and Secondary Cones in the Photoemission from a Real Solid
h6 Cqc}P 6.2.3 Angle-Integrated and Angle-Resolved Data Collection
:H>0/^Mg0 6.3 Photoemission from the Semi—infinite Crystal:The Inverse LEED Formalism
7'Gkip 6.3.1 Band Structure Regime
\WxBtpbQB 6.3.2 XPS Regime
gjn1ha"h%. 6.3.3 Surface Emission
Kiq[PK 6.3.4 One-Step Calculations
'3fN2[( 6.4 Thermal Effects
UdcrX`^. 6.5 Dipole Selection Rules for Direct Optical Transitions
i JS7g References
Z6 E_Y? $ EexNz 7.Band Structtire and Angular-Resolved Photoelectron Spectra
Nf%/)Tk 7.1 Free-Electron Final—State Model
Fb6d1I^wR 7.2 Methods Employing Calculated Band Structures
.+&M,%
x 7.3 Methods for the Absolute Determination of the Crystal Momentum
,O_iSohS 7.3.1 Triangulation or Energy Coincidence Method
{'yr)(:2M 7.3.2 Bragg Plane Method: Variation of External Emission Angle at Fixed Photon Frequency (Disappearance/Appearance Angle Method
+aN"*//i 7.3.3 Bragg Plane Method: Variation of Photon Energy at Fixed Emission Angle (Symmetry Method)
j7~Rw"(XQc 7.3.4 The Surface Emission Method and Electron Damping
t]E@AJOK 7.3.5 The Very-Low-Energy Electron Diffraction Method
:ZadPn56 7.3.6 The Fermi Surface Method
rUZ09>nDy 7.3.7 Intensities and Their Use in Band-Structure Determinations
P DwBSj 7.3.8 Summary
lr ]C'dD 7.4 Experimental Band Structures
%H4>k#b@$ 7.4.1 One- and Two-Dimensional Systems
^w_\D? 7.4.2 Three-Dimensional Solids: Metals and Semiconductors
KpT=twcK 7..4.3UPS Band Structures and XPS Density of States
DA>TT~L 7.5 A Comment
y7x*:xR[ References
r9n:[A&HE *gOUpbtXa 8.Surface States, Surface Effects
ydMSL25<+ 8.1 Theoretical Considerations
.$o
A~ 8.2 Experimental Results on Surface States
Ll, U>yo 8.3 Quantum-Well States
[DvQk?,t 8.4 Surface Core-Level Shifts
MqRJ:x References
/Ow@CB eVj7%9 9.Inverse Photoelectron Spectroscopy
KPA.5,ai 9.1 Surface States
*d9RD~Ee 9.2 Bulk Band Structures
~l]g4iEp 9.3 Adsorbed Molecules
hGRHuJ References
K94bM5O 1 -6$GM J7 10. Spin-Polarized Photoelectron Spectroscopy
38GZ_z}r 10.1 General Description
B_*Ayk
10.2 Examples of Spin-Polarized Photoelectron Spectroscopy
sfk;c#K 10.3 Magnetic Dichroism
9-!G Ya'Z References
bu{dT8g'U 9I(00t_ 11. Photoelectron Diffraction
~SS3gL v 11.1 Examples
klnk{R.>| 11.2 Substrate Photoelectron Diffraction
V3ExS1fNf 11.3 Adsorbate Photoelectron Diffraction
<u/(7H 11.4 Fermi Surface Scans
nPk&/H%5hn References
)r?-_qj= ?in)kL Appendix
D"exI] A.1 Table of Binding Energies
QOY{j A.2 Surface and Bulk Brillouin Zones of the Three Low-Index Faces of a Face—Centered Cubic(fcc)Crystal Face
EI496bsRHm A.3 Compilation of Work Functions
hD{
`j References
R?M>uaxn Index