光电子谱技术是研究原子、分子、固体和表面电子
结构的一种非常有效的手段。本书全面
系统地介绍了
光电子谱技术的
原理和应用,并简明讨论了逆光发射、自旋极化光发射和
光电子衍射等现象。本书是一本非常实用的光电子谱技术的专著,内容几乎覆盖了光电子研究的所有领域。其特点是紧密联系实验,并利用理论详细解释实验结果,达到理论和应用的有机结合。书中还收集了大量的实际
材料的光电子谱分析,同时给出了大量的实验数据,以便于读者的查阅。总之,该书既是一本很有价值的参考书,又可作为初学者的入门教材。
J3y4D} ]SL0Mn g8 作者在该领域做出了杰出的贡献。在第3版中,作者介绍了大量最新研究成果,并对光电子谱技术很多方面给出了有深刻见解的讨论。
J0UF( H'?dsc 读者对象:适用于凝聚态
物理学、材料物理学和光电子学等专业的高年级本科生、研究生和相关专业的科研人员。
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Y))x'<T'Q h 6juX'V 目录
p9gX$-!pbG 1. Introduction and Basic Principles
LfX[(FP 1.1 Historical Development
Rv|X\Wm 1.2 The Electron Mean Free Path
6tN!] 1.3 Photoelectron Spectroscopy and Inverse Photoelectron Spectroscopy
=j~Xrytn 1.4 Experimental Aspects
C%Fc%}[ 1.5 Very High Resolution
aH*5(E] 1.6 The Theory of Photoemission
aK]H(F2# 1.6.1 Core-Level Photoemission
]L_h3Xz\X 1.6.2 Valence-State Photoemission
RP%7M8V){B 1.6.3 Three-Step and One-Step Considerations
wqAj=1M\ 1.7 Deviations from the Simple Theory of Photoemission
dCO)"] References
sW0<f&3 ?y2v?h" 2. Core Levels and Final States
fvr|<3ojo 2.1 Core-Level Binding Energies in Atoms and Molecules
q]wP^;\Jl 2.1.1 The Equivalent-Core Approximation
`Zd\d:Wyv 2.1.2 Chemical Shifts
t&H3yV 2.2 Core-Level Binding Energies in Solids
?btZdnQ))S 2.2.1 The Born-Haber Cycle in Insulators
Iz9b5 2.2.2 Theory of Binding Energies
G'(8/os{ 2.2.3 Determination of Binding Energies and Chemical Shifts from Thermodynamic Data
,_I#+XiXY 2.3 Core Polarization
E\vW>g*W 2.4 Final-State Multiplets in Rare-Earth Valence Bands
A x'o|RE)x 2.5 Vibrational Side Bands
66|$X, 2.6 Core Levels of Adsorbed Molecules
4+q3
Kw 2.7 Quantitative Chemical Analysis from Core-Level Intensities
|`Iispn References
yc.9CTxx o|nN0z)b4 3. Charge-Excitation Final States: Satellites
_qsg2e}n 3.1 Copper Dihalides; 3d Transition Metal Compounds
X^)vZL? 3.1.1 Characterization of a Satellite
L[O.]2 3.1.2 Analysis of Charge-Transfer Satellites
D}]u9jS1 3.1.3 Non-local Screening
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$9eK@ 3.2 The 6-eV Satellite in Nickel
D0LoT?$N 3.2.1 Resonance Photoemission
!EB[Lutm 3.2.2 Satellites in Other Metals
%>EM ^Z 3.3 The Gunnarsson-Sch6nhammer Theory
?VR:e7|tU 3.4 Photoemission Signals and Narrow Bands in Metals
M7\yEi"* References
y\zRv(T= i]}`e>fF 4. Continuous Satellites and Plasmon Satellites: XPS Photoemission in Nearly Free Electron Systems
1[ 40\ sM 4.1 Theory
@h!nVf%fe 4.1.1 General
G }U'?p 4.1.2 Core-Line Shape
E{xcu9 4.1.3 Intrinsic Plasmons
KLCd`vr.xf 4.1.4 Fxtrinsic FAectron Scattering: Plasmons and Background
48RSuH 4.1.5 The Total Photoelectron Spectrum
>WmTM0 4.2 Experimental Results
s|IC;C| 4.2.1 The Core Line Without Plasmons
XY!0yAK(! 4.2.2 Core-Level Spectra Including Plasmoas
eWWfUNBSLX 4.2.3 Valence-Band Spectra of the Simple Metals
wOF";0EN 4.2.4 Simple Metals: A General Comment
)=%TIkeF 4.3 The Background Correction
\7] SG References
i2X%xYv ^ tWaM+W 5. Valence Orbitals in Simple Molecules and Insulating Solids
'oS= d 5.1 UPS Spectra of Monatomic Gases
}N0v_Nas;v 5.2 Photoelectron Spectra of Diatomic Molecules
bL0>ul" 5.3 Binding Energy of the H2 Molecule
NM4b]> 5.4 Hydrides Isoelectronic with Noble Gases
ayrCLv Neon (Ne)
`XrF , Hydrogen Fluoride (HF)
+\U#:gmw Water (H2O)
.dKFQH iYJ Ammonia (NH3)
Xhp={p; Methane (CH4)
# "!q_@b,D 5.5 Spectra of the Alkali HMides
Q|(G - 5.6 Transition Metal Dihalides
\`Ow)t: 5.7 Hydrocarbons
Ft 6{g
JBG 5.7.1 Guidelines for the Interpretation of Spectra from Free Molecules
q.!<GqSgb 5.7.2 Linear Polymers
DE!c+s_g4 5.8 Insulating Solids with Valence d Electrons
`%Dz 8Z 5.8.1 The NiO Problem
+jb<=ERV[ 5.8.2 Mort Insulation
Y>Fh<"A|$ 5.8.3 The Metal-Insulator Transition;the Ratio of the Correlation Energy and the Bandwidth;Doping
0F9p'_C 5.8.4Band Structures of Transition Metal Compounds
%![3?|8~ 5.9 High—Temperature Superconductors
,racmxnv 5.9.1valence-Band Electronic Structure;Polycrystalline Samples
>b2wFo/em 5.9.2 Dispersion Relations in High Temperature Superconductors;Single Crystals
^0HgE;4 5.9.3 The Superconducting Gap
!yD$fY 5.9.4 Symmetry of the Order Parameter in the High-Temperature SuDerconductors
`&URd&ouJD 5.9.5 Core—Level Shifts
^=[b]*V 5.10 The Fermi Liquid and the Luttinger Liquid
/Suh&qw>
5.11 Adsorbed Molecules
:N64FR# 5.11.1 Outline
85qD~o?O 5.11.2 CO on Metal Surfaces
C9^C4
References
i)=
\-C Q/`W[Et 6.Photoemission of Valence Electrons froill Metallic Solids in the OHe-Electron Approximation
`Jn2(+ 6.1 Theory of Photoemission:A Summary of the Three-Step Model
/@Ec[4^=!. 6.2 Discussion of the Photocurrent
Cq[<CPAS 6.2.1 Kinematics of Internal Photoemission in a Polycrystalline Sample
s2"<<P[q' 6.2.2 Primary and Secondary Cones in the Photoemission from a Real Solid
7UsU03 6.2.3 Angle-Integrated and Angle-Resolved Data Collection
5+[ 3@ 6.3 Photoemission from the Semi—infinite Crystal:The Inverse LEED Formalism
`Ha<t. v( 6.3.1 Band Structure Regime
N"A`tc5& 6.3.2 XPS Regime
6)yi^v 6.3.3 Surface Emission
2:G/Oj h&] 6.3.4 One-Step Calculations
qaG8: 6.4 Thermal Effects
p(.z#o# 6.5 Dipole Selection Rules for Direct Optical Transitions
dfT References
uU/'oZ? -8Hv3J'= 7.Band Structtire and Angular-Resolved Photoelectron Spectra
#+L:V&QE 7.1 Free-Electron Final—State Model
A,4Z{f83 7.2 Methods Employing Calculated Band Structures
+g&M@8XO& 7.3 Methods for the Absolute Determination of the Crystal Momentum
Xxr"Gc[ 7.3.1 Triangulation or Energy Coincidence Method
7gE/g`"# 7.3.2 Bragg Plane Method: Variation of External Emission Angle at Fixed Photon Frequency (Disappearance/Appearance Angle Method
EIF"{,m 7.3.3 Bragg Plane Method: Variation of Photon Energy at Fixed Emission Angle (Symmetry Method)
nQ#NW8*Fs 7.3.4 The Surface Emission Method and Electron Damping
.4[M7) 7.3.5 The Very-Low-Energy Electron Diffraction Method
zg$NrI& 7.3.6 The Fermi Surface Method
Axw+zO 7.3.7 Intensities and Their Use in Band-Structure Determinations
,j(S'Pw 7.3.8 Summary
@ \*Zq 7.4 Experimental Band Structures
6"yIk4u: 7.4.1 One- and Two-Dimensional Systems
Yc^,Cj{OM 7.4.2 Three-Dimensional Solids: Metals and Semiconductors
y wmC>`0p 7..4.3UPS Band Structures and XPS Density of States
/YHnt-}v, 7.5 A Comment
z@[-+Q: References
h-6x! 6pm !q 9PO 8.Surface States, Surface Effects
$0*D7P^8 8.1 Theoretical Considerations
t8.^Y TI 8.2 Experimental Results on Surface States
O% 8>siU 8.3 Quantum-Well States
kL"Y>@H 8.4 Surface Core-Level Shifts
~p
x2kHZ References
,L\>mGw #N'bhs 9.Inverse Photoelectron Spectroscopy
EN5F*s@r 9.1 Surface States
S]?I7_ 9.2 Bulk Band Structures
('+C $ 9.3 Adsorbed Molecules
cH6J:0>W References
~cSE 9ul b1EY6'R2 10. Spin-Polarized Photoelectron Spectroscopy
K_%gda|l+ 10.1 General Description
oB+Ek~{z] 10.2 Examples of Spin-Polarized Photoelectron Spectroscopy
|%@pjJ`3 10.3 Magnetic Dichroism
DDe`Lb%% References
0~BZh%s< ( nw0Tg= P 11. Photoelectron Diffraction
O@a7MzJ 11.1 Examples
C);I[H4Yfw 11.2 Substrate Photoelectron Diffraction
{J-Ojw|Y b 11.3 Adsorbate Photoelectron Diffraction
i93^E~q] 11.4 Fermi Surface Scans
EZ[e
a< References
KebC$g@W f1q0*)fk Appendix
_|7bpt9 A.1 Table of Binding Energies
0+NGFX\p A.2 Surface and Bulk Brillouin Zones of the Three Low-Index Faces of a Face—Centered Cubic(fcc)Crystal Face
cUTG!
P\R A.3 Compilation of Work Functions
{T 3~js References
I "HEXsSe Index