光电子谱技术是研究原子、分子、固体和表面电子
结构的一种非常有效的手段。本书全面
系统地介绍了
光电子谱技术的
原理和应用,并简明讨论了逆光发射、自旋极化光发射和
光电子衍射等现象。本书是一本非常实用的光电子谱技术的专著,内容几乎覆盖了光电子研究的所有领域。其特点是紧密联系实验,并利用理论详细解释实验结果,达到理论和应用的有机结合。书中还收集了大量的实际
材料的光电子谱分析,同时给出了大量的实验数据,以便于读者的查阅。总之,该书既是一本很有价值的参考书,又可作为初学者的入门教材。
wr{ [4$O w</qUOx 作者在该领域做出了杰出的贡献。在第3版中,作者介绍了大量最新研究成果,并对光电子谱技术很多方面给出了有深刻见解的讨论。
[rf.& >cYYr@S 读者对象:适用于凝聚态
物理学、材料物理学和光电子学等专业的高年级本科生、研究生和相关专业的科研人员。
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`%nj$-W: j$mCU? 目录
e3!0<A[X 1. Introduction and Basic Principles
hUO&rov3@ 1.1 Historical Development
B>XfsZS 1.2 The Electron Mean Free Path
q{E44
eQ7F 1.3 Photoelectron Spectroscopy and Inverse Photoelectron Spectroscopy
GiGXV @dq 1.4 Experimental Aspects
RI</T3%~ 1.5 Very High Resolution
(// f"c]/ 1.6 The Theory of Photoemission
\;F_QV 1.6.1 Core-Level Photoemission
}V I}O{ 1.6.2 Valence-State Photoemission
5*P+c(= 1.6.3 Three-Step and One-Step Considerations
0kOl,%Ey 1.7 Deviations from the Simple Theory of Photoemission
>J,y1jzJ References
v[J"/:] e_Un:r@) 2. Core Levels and Final States
m2h@* 2.1 Core-Level Binding Energies in Atoms and Molecules
6tKCY(#oO+ 2.1.1 The Equivalent-Core Approximation
<yw(7 2.1.2 Chemical Shifts
{Xw6p 2.2 Core-Level Binding Energies in Solids
gSn9L)k(O 2.2.1 The Born-Haber Cycle in Insulators
SoPiEq 2.2.2 Theory of Binding Energies
{M&Vh] 2.2.3 Determination of Binding Energies and Chemical Shifts from Thermodynamic Data
i?0+f}5<p 2.3 Core Polarization
rwh,RI)
)g 2.4 Final-State Multiplets in Rare-Earth Valence Bands
KYN{Dh]-} 2.5 Vibrational Side Bands
RP|/rd]-k 2.6 Core Levels of Adsorbed Molecules
-H-:b7 2.7 Quantitative Chemical Analysis from Core-Level Intensities
roNRbA] References
3d81]!n X+LG Z4]D 3. Charge-Excitation Final States: Satellites
+2?=W1` 3.1 Copper Dihalides; 3d Transition Metal Compounds
qOM" ?av 3.1.1 Characterization of a Satellite
6L}}3b h 3.1.2 Analysis of Charge-Transfer Satellites
S#{gCc 3.1.3 Non-local Screening
<A+n[h 3.2 The 6-eV Satellite in Nickel
7ea<2va, 3.2.1 Resonance Photoemission
BK;Gh0mp 3.2.2 Satellites in Other Metals
_ 0g\g~[ 3.3 The Gunnarsson-Sch6nhammer Theory
>A_:qyGk 3.4 Photoemission Signals and Narrow Bands in Metals
_G0_<WH6 References
yNc"E
XMpa87\ 4. Continuous Satellites and Plasmon Satellites: XPS Photoemission in Nearly Free Electron Systems
%TUvH>;0 4.1 Theory
r)xkpa5 4.1.1 General
O}w"@gO@. 4.1.2 Core-Line Shape
HmQ.' 4.1.3 Intrinsic Plasmons
.,+TpPkc 4.1.4 Fxtrinsic FAectron Scattering: Plasmons and Background
K}e:zR;;^ 4.1.5 The Total Photoelectron Spectrum
&Ay[mZQ 7 4.2 Experimental Results
'ugc=-0pd 4.2.1 The Core Line Without Plasmons
CaE1h9 4.2.2 Core-Level Spectra Including Plasmoas
/|MHZ$Y9w? 4.2.3 Valence-Band Spectra of the Simple Metals
\{u 9Kc 4.2.4 Simple Metals: A General Comment
/;{E}` 4.3 The Background Correction
l>){cI/D# References
56`Tna,t x,81#=m^h 5. Valence Orbitals in Simple Molecules and Insulating Solids
L5j%4BlK/ 5.1 UPS Spectra of Monatomic Gases
=&~7Q" 5.2 Photoelectron Spectra of Diatomic Molecules
c+A$ [ 5.3 Binding Energy of the H2 Molecule
kfj)`x 5.4 Hydrides Isoelectronic with Noble Gases
uw>O|&! Neon (Ne)
p'f8?jt Hydrogen Fluoride (HF)
=9yh<'583 Water (H2O)
oqUF_kh Ammonia (NH3)
CyXFuk!R Methane (CH4)
,$A'Y 5.5 Spectra of the Alkali HMides
}p|S3/G?$! 5.6 Transition Metal Dihalides
bo|3sN+D 5.7 Hydrocarbons
iKM!>Fi 5.7.1 Guidelines for the Interpretation of Spectra from Free Molecules
>K;DBy* 5.7.2 Linear Polymers
a2%xW_e 5.8 Insulating Solids with Valence d Electrons
BL[N 5.8.1 The NiO Problem
?%A9}"q] 5.8.2 Mort Insulation
kWMz;{I5*w 5.8.3 The Metal-Insulator Transition;the Ratio of the Correlation Energy and the Bandwidth;Doping
fPBJ%SZ 5.8.4Band Structures of Transition Metal Compounds
U]A JWC6 5.9 High—Temperature Superconductors
"zZZ h 5.9.1valence-Band Electronic Structure;Polycrystalline Samples
j/p1/sJ[y 5.9.2 Dispersion Relations in High Temperature Superconductors;Single Crystals
!*G%vOa 5.9.3 The Superconducting Gap
N5d)&a
7? 5.9.4 Symmetry of the Order Parameter in the High-Temperature SuDerconductors
RIdh],- 5.9.5 Core—Level Shifts
s~'"&0Gz 5.10 The Fermi Liquid and the Luttinger Liquid
4^(aG7 5.11 Adsorbed Molecules
FKBI.}A?!' 5.11.1 Outline
VSjt|F)t 5.11.2 CO on Metal Surfaces
f"RS,] References
H ]z83:Z ;_p$5GVR| 6.Photoemission of Valence Electrons froill Metallic Solids in the OHe-Electron Approximation
Rl{e<>O\^ 6.1 Theory of Photoemission:A Summary of the Three-Step Model
i z%wozf 6.2 Discussion of the Photocurrent
<q.Q,_cW 6.2.1 Kinematics of Internal Photoemission in a Polycrystalline Sample
/
DG t 6.2.2 Primary and Secondary Cones in the Photoemission from a Real Solid
=n<Lbl(7 6.2.3 Angle-Integrated and Angle-Resolved Data Collection
c:I %jm 6.3 Photoemission from the Semi—infinite Crystal:The Inverse LEED Formalism
38#Zlcf 6.3.1 Band Structure Regime
u*=8s5Q[ 6.3.2 XPS Regime
!rsGCw!Pg 6.3.3 Surface Emission
nq5qUErew 6.3.4 One-Step Calculations
JnIE6@g<y 6.4 Thermal Effects
J!\oH%FJp 6.5 Dipole Selection Rules for Direct Optical Transitions
XY^]nm-{I References
.]w=+~h .+(R,SvN%< 7.Band Structtire and Angular-Resolved Photoelectron Spectra
^D8~s; ? 7.1 Free-Electron Final—State Model
'\M]$`Et 7.2 Methods Employing Calculated Band Structures
alH6~ 7.3 Methods for the Absolute Determination of the Crystal Momentum
?[<#>,W 7.3.1 Triangulation or Energy Coincidence Method
cDIZkni= 7.3.2 Bragg Plane Method: Variation of External Emission Angle at Fixed Photon Frequency (Disappearance/Appearance Angle Method
FDal;T
7.3.3 Bragg Plane Method: Variation of Photon Energy at Fixed Emission Angle (Symmetry Method)
+Ly@5y" 7.3.4 The Surface Emission Method and Electron Damping
Ge7Uety 7.3.5 The Very-Low-Energy Electron Diffraction Method
Vbv)C3ezD 7.3.6 The Fermi Surface Method
HA74s':FN 7.3.7 Intensities and Their Use in Band-Structure Determinations
*7o@HBbF 7.3.8 Summary
p""\uG' 7.4 Experimental Band Structures
T5Iz{Ha 7.4.1 One- and Two-Dimensional Systems
H/U.Bg 4 7.4.2 Three-Dimensional Solids: Metals and Semiconductors
bae;2| w 7..4.3UPS Band Structures and XPS Density of States
6Ts[NXa 7.5 A Comment
=m;,?("7t3 References
<?>tjCg' A{p_I< 8.Surface States, Surface Effects
Cto>~pV 8.1 Theoretical Considerations
GTM@9^ 8.2 Experimental Results on Surface States
zY9CoadZ 8.3 Quantum-Well States
h
S)lQl:^ 8.4 Surface Core-Level Shifts
z HT#bP:o References
x[=,$;o+ E7q,6f3@r 9.Inverse Photoelectron Spectroscopy
*ze,X~8- 9.1 Surface States
y$+=>p|d.^ 9.2 Bulk Band Structures
Re+oCJ 9.3 Adsorbed Molecules
22'Ra[ References
DwGRv:&HH U+R9bn 10. Spin-Polarized Photoelectron Spectroscopy
U(gYx@ 10.1 General Description
=QK ucLo 10.2 Examples of Spin-Polarized Photoelectron Spectroscopy
Rl&nR$# 10.3 Magnetic Dichroism
NL,6<ZOon, References
G.r .Z0 NxSSRv^rx 11. Photoelectron Diffraction
Y-lwS-Ii 11.1 Examples
#jJ0Mxg 11.2 Substrate Photoelectron Diffraction
MOPHu
O{^ 11.3 Adsorbate Photoelectron Diffraction
%l,CJd5 11.4 Fermi Surface Scans
`A9fanh References
w
_4O; _Wq;bKG Appendix
5=\^DeM@
H A.1 Table of Binding Energies
V qcw2 A.2 Surface and Bulk Brillouin Zones of the Three Low-Index Faces of a Face—Centered Cubic(fcc)Crystal Face
&kcmkRRG A.3 Compilation of Work Functions
'P*OzZ4>$ References
T% GR{mp Index