光电子谱技术是研究原子、分子、固体和表面电子
结构的一种非常有效的手段。本书全面
系统地介绍了
光电子谱技术的
原理和应用,并简明讨论了逆光发射、自旋极化光发射和
光电子衍射等现象。本书是一本非常实用的光电子谱技术的专著,内容几乎覆盖了光电子研究的所有领域。其特点是紧密联系实验,并利用理论详细解释实验结果,达到理论和应用的有机结合。书中还收集了大量的实际
材料的光电子谱分析,同时给出了大量的实验数据,以便于读者的查阅。总之,该书既是一本很有价值的参考书,又可作为初学者的入门教材。
]c~yMA+]FZ vMB61 |O 作者在该领域做出了杰出的贡献。在第3版中,作者介绍了大量最新研究成果,并对光电子谱技术很多方面给出了有深刻见解的讨论。
o0]YDX@T "qNFDr(WM 读者对象:适用于凝聚态
物理学、材料物理学和光电子学等专业的高年级本科生、研究生和相关专业的科研人员。
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P*A+k"DU1
*{vH9TO Ig t*8px 目录
s`_EkFw>Gl 1. Introduction and Basic Principles
Q $}#& 1.1 Historical Development
aWIkp5BFj 1.2 The Electron Mean Free Path
_i}b]xfM 1.3 Photoelectron Spectroscopy and Inverse Photoelectron Spectroscopy
6qHD&bv\%C 1.4 Experimental Aspects
zPa2fS8 1.5 Very High Resolution
3"7Q[9Oj 1.6 The Theory of Photoemission
e{@RBYX@+c 1.6.1 Core-Level Photoemission
<7VLUk} 1.6.2 Valence-State Photoemission
?@9v+Am! 1.6.3 Three-Step and One-Step Considerations
ANFes*8j 1.7 Deviations from the Simple Theory of Photoemission
pOXI*0_g. References
U-9Aq NgDhdOB 2. Core Levels and Final States
ywAvqT, 2.1 Core-Level Binding Energies in Atoms and Molecules
ID2->J 2.1.1 The Equivalent-Core Approximation
U
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B18BwY 2.2 Core-Level Binding Energies in Solids
SG)Fk *1 2.2.1 The Born-Haber Cycle in Insulators
j|[rT^b@ 2.2.2 Theory of Binding Energies
q$:7j5E 2.2.3 Determination of Binding Energies and Chemical Shifts from Thermodynamic Data
{6v.(Zlh$ 2.3 Core Polarization
`!vqT 3p, 2.4 Final-State Multiplets in Rare-Earth Valence Bands
YWK0.F,8a 2.5 Vibrational Side Bands
b^$`2m-?@f 2.6 Core Levels of Adsorbed Molecules
bW6| &P}X 2.7 Quantitative Chemical Analysis from Core-Level Intensities
D<6$@ZJ References
E+lR&~mK= x(TF4W=j 3. Charge-Excitation Final States: Satellites
IQPu%n{0v 3.1 Copper Dihalides; 3d Transition Metal Compounds
,Q-,#C" 3.1.1 Characterization of a Satellite
iAk:CJ{ 3.1.2 Analysis of Charge-Transfer Satellites
hn8xs5vN 3.1.3 Non-local Screening
7HDc]&z 3.2 The 6-eV Satellite in Nickel
x#EE_i/W 3.2.1 Resonance Photoemission
$&as5z8 3.2.2 Satellites in Other Metals
|reA`&<q 3.3 The Gunnarsson-Sch6nhammer Theory
;
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o99ExQ. References
fEZuv?@ L;RE5YrH%6 4. Continuous Satellites and Plasmon Satellites: XPS Photoemission in Nearly Free Electron Systems
~#sD2b`0 4.1 Theory
/aI@2] |~ 4.1.1 General
\#HW.5 4.1.2 Core-Line Shape
[[ie 4.1.3 Intrinsic Plasmons
&s+l/;3 4.1.4 Fxtrinsic FAectron Scattering: Plasmons and Background
[A7TSN 4.1.5 The Total Photoelectron Spectrum
$xWwI(SaB 4.2 Experimental Results
idYB.]Y( 4.2.1 The Core Line Without Plasmons
3J#LxYK 4.2.2 Core-Level Spectra Including Plasmoas
7%Y`j/ 4.2.3 Valence-Band Spectra of the Simple Metals
.G[/4h :. 4.2.4 Simple Metals: A General Comment
^aSb~lce 4.3 The Background Correction
YCbvCw$Ob References
!q2zuxq!R B>fZH\Y 5. Valence Orbitals in Simple Molecules and Insulating Solids
!zX()V
5.1 UPS Spectra of Monatomic Gases
%
"(&a'B 5.2 Photoelectron Spectra of Diatomic Molecules
F@u7Oel@m 5.3 Binding Energy of the H2 Molecule
4aS}b3=n 5.4 Hydrides Isoelectronic with Noble Gases
$X#y9<bW Neon (Ne)
*]]Zpa6 Hydrogen Fluoride (HF)
spV7\Gs.@ Water (H2O)
j L|6i-?! Ammonia (NH3)
.g8*K " Methane (CH4)
4-yK!LR 5.5 Spectra of the Alkali HMides
L!cOg8Z 5.6 Transition Metal Dihalides
"N}t =3i$ 5.7 Hydrocarbons
j}^w:W76 5.7.1 Guidelines for the Interpretation of Spectra from Free Molecules
%y RGN 5.7.2 Linear Polymers
?@ oF@AEx= 5.8 Insulating Solids with Valence d Electrons
X<%D@$ 5.8.1 The NiO Problem
/pj[c;aO 5.8.2 Mort Insulation
v&d1ACctJ 5.8.3 The Metal-Insulator Transition;the Ratio of the Correlation Energy and the Bandwidth;Doping
'#+&?6 p 5.8.4Band Structures of Transition Metal Compounds
Z mJ<h& 5.9 High—Temperature Superconductors
p / ITg 5.9.1valence-Band Electronic Structure;Polycrystalline Samples
[Z$H<m{c- 5.9.2 Dispersion Relations in High Temperature Superconductors;Single Crystals
iJzBd7 5.9.3 The Superconducting Gap
%zcA|SefP 5.9.4 Symmetry of the Order Parameter in the High-Temperature SuDerconductors
VE+H! ob
A 5.9.5 Core—Level Shifts
h$02#(RHJ 5.10 The Fermi Liquid and the Luttinger Liquid
~&<#H+O 5.11 Adsorbed Molecules
*BsK6iVb 5.11.1 Outline
-uYxc=4Lh 5.11.2 CO on Metal Surfaces
UMGiJO\yH References
VhO%4[Jl g+#awi7 6.Photoemission of Valence Electrons froill Metallic Solids in the OHe-Electron Approximation
MKBDWLCB 6.1 Theory of Photoemission:A Summary of the Three-Step Model
&&&-P\3 6.2 Discussion of the Photocurrent
+u$l]~St\ 6.2.1 Kinematics of Internal Photoemission in a Polycrystalline Sample
I){4MoH. 6.2.2 Primary and Secondary Cones in the Photoemission from a Real Solid
D>7a0p784 6.2.3 Angle-Integrated and Angle-Resolved Data Collection
b}K,wAx
6.3 Photoemission from the Semi—infinite Crystal:The Inverse LEED Formalism
`==l2AX 6.3.1 Band Structure Regime
cwmS4^zt8 6.3.2 XPS Regime
q}LDFsU 6.3.3 Surface Emission
.ck?JXg 6.3.4 One-Step Calculations
gQeQy 6.4 Thermal Effects
E.K^v/dNdq 6.5 Dipole Selection Rules for Direct Optical Transitions
EOB8|:* References
zy,SL
|6: a}UmD
HS- 7.Band Structtire and Angular-Resolved Photoelectron Spectra
\|,| ) 7.1 Free-Electron Final—State Model
;C@mT;hR 7.2 Methods Employing Calculated Band Structures
1=)M15 7.3 Methods for the Absolute Determination of the Crystal Momentum
*JJ8\R&P0 7.3.1 Triangulation or Energy Coincidence Method
'9}&@;-_ 7.3.2 Bragg Plane Method: Variation of External Emission Angle at Fixed Photon Frequency (Disappearance/Appearance Angle Method
{'IO 7.3.3 Bragg Plane Method: Variation of Photon Energy at Fixed Emission Angle (Symmetry Method)
g{'f%bkG 7.3.4 The Surface Emission Method and Electron Damping
'7?Y+R@|L 7.3.5 The Very-Low-Energy Electron Diffraction Method
DB|1Sqjsn 7.3.6 The Fermi Surface Method
:H]d1 7.3.7 Intensities and Their Use in Band-Structure Determinations
(ghI$oH 7.3.8 Summary
r9ulTv}X 7.4 Experimental Band Structures
]hS:0QE 7.4.1 One- and Two-Dimensional Systems
yNI0Do
2 7.4.2 Three-Dimensional Solids: Metals and Semiconductors
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7..4.3UPS Band Structures and XPS Density of States
'[#y| 7.5 A Comment
uPfz'|, References
~q ^o|? \;&;K'
8.Surface States, Surface Effects
=|?`5!A 8.1 Theoretical Considerations
;E.]:Ia~ 8.2 Experimental Results on Surface States
_LaG%* R6 8.3 Quantum-Well States
%/A>'p,~ 8.4 Surface Core-Level Shifts
c>LP}PGk References
EVPQe- 5MnP6(3$ 9.Inverse Photoelectron Spectroscopy
UePkSz9EU 9.1 Surface States
Jpapl%7v 9.2 Bulk Band Structures
l eC!Yj 9.3 Adsorbed Molecules
E
f\|3D_ References
|]< 3cW+ x9 > ho 10. Spin-Polarized Photoelectron Spectroscopy
R%jOgZG 10.1 General Description
tW UI?\ 10.2 Examples of Spin-Polarized Photoelectron Spectroscopy
s;vt2>;q+e 10.3 Magnetic Dichroism
NW[K/`-CTH References
NVMn7H}>
Qf~>5(,h 11. Photoelectron Diffraction
bWo 11.1 Examples
H^-Y]{7 11.2 Substrate Photoelectron Diffraction
Eg)24C R 4 11.3 Adsorbate Photoelectron Diffraction
z 206fF 11.4 Fermi Surface Scans
l2LQV]l References
NTu|cX\R Al^tM0T^ Appendix
c]M+|R5 A.1 Table of Binding Energies
({E,}x A.2 Surface and Bulk Brillouin Zones of the Three Low-Index Faces of a Face—Centered Cubic(fcc)Crystal Face
> Z+*tq A.3 Compilation of Work Functions
$]DuO1H./ References
@\g}I`_M Index