光电子谱技术是研究原子、分子、固体和表面电子
结构的一种非常有效的手段。本书全面
系统地介绍了
光电子谱技术的
原理和应用,并简明讨论了逆光发射、自旋极化光发射和
光电子衍射等现象。本书是一本非常实用的光电子谱技术的专著,内容几乎覆盖了光电子研究的所有领域。其特点是紧密联系实验,并利用理论详细解释实验结果,达到理论和应用的有机结合。书中还收集了大量的实际
材料的光电子谱分析,同时给出了大量的实验数据,以便于读者的查阅。总之,该书既是一本很有价值的参考书,又可作为初学者的入门教材。
X @r5^A[9 =d(
6
) 作者在该领域做出了杰出的贡献。在第3版中,作者介绍了大量最新研究成果,并对光电子谱技术很多方面给出了有深刻见解的讨论。
I"Y?vj9] iTxn 读者对象:适用于凝聚态
物理学、材料物理学和光电子学等专业的高年级本科生、研究生和相关专业的科研人员。
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*/?L_\7 NE3G!qxL 目录
`p'L3u5H- 1. Introduction and Basic Principles
WET $H, 1.1 Historical Development
/WMG)#kw' 1.2 The Electron Mean Free Path
dI'C[.zp[ 1.3 Photoelectron Spectroscopy and Inverse Photoelectron Spectroscopy
uK): d&]Ux 1.4 Experimental Aspects
y 0M&Bh 1.5 Very High Resolution
6U# C
1.6 The Theory of Photoemission
zKgW9j<( 1.6.1 Core-Level Photoemission
[yjC@docH 1.6.2 Valence-State Photoemission
@WFjM 1.6.3 Three-Step and One-Step Considerations
`4Nc(aUr 1.7 Deviations from the Simple Theory of Photoemission
[y>Q3UqN References
cCWOGd
s9O] tk 2. Core Levels and Final States
Fv e,&~ 2.1 Core-Level Binding Energies in Atoms and Molecules
qF( ]Ce 2.1.1 The Equivalent-Core Approximation
h7(twct 2.1.2 Chemical Shifts
7|65;jm+ 2.2 Core-Level Binding Energies in Solids
EYG&~a>L* 2.2.1 The Born-Haber Cycle in Insulators
IcaIB) 2.2.2 Theory of Binding Energies
^!Bpev 2.2.3 Determination of Binding Energies and Chemical Shifts from Thermodynamic Data
$W`
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N9{ivq|fO 2.4 Final-State Multiplets in Rare-Earth Valence Bands
v-OGY[|97 2.5 Vibrational Side Bands
nLT]'B]$+ 2.6 Core Levels of Adsorbed Molecules
2NE/ZqREg 2.7 Quantitative Chemical Analysis from Core-Level Intensities
_H:SoJ' References
5nf|CQH6? BWw7o{d 3. Charge-Excitation Final States: Satellites
_FAwW<S4B 3.1 Copper Dihalides; 3d Transition Metal Compounds
bFJmXx& 3.1.1 Characterization of a Satellite
L\hPw{) 3.1.2 Analysis of Charge-Transfer Satellites
%'^m6^g; 3.1.3 Non-local Screening
RTF{<,E.UX 3.2 The 6-eV Satellite in Nickel
REFisH- 3.2.1 Resonance Photoemission
l 4~'CLi 3.2.2 Satellites in Other Metals
zA( 2+e 7 3.3 The Gunnarsson-Sch6nhammer Theory
V@cRJ3ZF 3.4 Photoemission Signals and Narrow Bands in Metals
V 9=y@`; References
eb.`Q+Gb y "7TO# 4. Continuous Satellites and Plasmon Satellites: XPS Photoemission in Nearly Free Electron Systems
^_2Ki 4.1 Theory
?e&CbVc4 4.1.1 General
oJXZ}>>iT 4.1.2 Core-Line Shape
L~vNW6#W 4.1.3 Intrinsic Plasmons
,{zvGZ| 4.1.4 Fxtrinsic FAectron Scattering: Plasmons and Background
Z AZQFr'* 4.1.5 The Total Photoelectron Spectrum
XXe7w3x{ 4.2 Experimental Results
S7N54X2JwL 4.2.1 The Core Line Without Plasmons
)
e;F@o3 4.2.2 Core-Level Spectra Including Plasmoas
nJ2l$J< 4.2.3 Valence-Band Spectra of the Simple Metals
U.>n]/& 4.2.4 Simple Metals: A General Comment
rr9HC]63 4.3 The Background Correction
Q5 ohaxjF References
E7*1QR{Q eaF5S'k 4$ 5. Valence Orbitals in Simple Molecules and Insulating Solids
Wy4v~]xd% 5.1 UPS Spectra of Monatomic Gases
EcwHO 5.2 Photoelectron Spectra of Diatomic Molecules
|bd5aRS9 5.3 Binding Energy of the H2 Molecule
?]5wX2G^|J 5.4 Hydrides Isoelectronic with Noble Gases
^Ko0zz|R/ Neon (Ne)
<NS=<'U Hydrogen Fluoride (HF)
=PO/Q|-v? Water (H2O)
\6C"bQ Ammonia (NH3)
*%8,G'"r? Methane (CH4)
(v(_XlMK 5.5 Spectra of the Alkali HMides
XUMCz7&j 5.6 Transition Metal Dihalides
D8Ni=.ALL 5.7 Hydrocarbons
*OsXjL`f 5.7.1 Guidelines for the Interpretation of Spectra from Free Molecules
qZ8lU 5.7.2 Linear Polymers
|wK)(s 5.8 Insulating Solids with Valence d Electrons
TR
]lP<m 5.8.1 The NiO Problem
14zo0ANM 5.8.2 Mort Insulation
c}rRNS$F 5.8.3 The Metal-Insulator Transition;the Ratio of the Correlation Energy and the Bandwidth;Doping
a&Z|3+ZA 5.8.4Band Structures of Transition Metal Compounds
sH+]lTSX6{ 5.9 High—Temperature Superconductors
QuF%m^aE 5.9.1valence-Band Electronic Structure;Polycrystalline Samples
#Oe=G:+A 5.9.2 Dispersion Relations in High Temperature Superconductors;Single Crystals
U/jJ@8 5.9.3 The Superconducting Gap
LM*9b 5.9.4 Symmetry of the Order Parameter in the High-Temperature SuDerconductors
gs0,-) 5.9.5 Core—Level Shifts
>@ EQarD 5.10 The Fermi Liquid and the Luttinger Liquid
>1joCG~ 5.11 Adsorbed Molecules
9rA3qj% 5.11.1 Outline
FK
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%f:'A%'Qb References
gvsS:4N"Nq urtcSq&H' 6.Photoemission of Valence Electrons froill Metallic Solids in the OHe-Electron Approximation
(<8T*Xo 6.1 Theory of Photoemission:A Summary of the Three-Step Model
?w<x_Lo 6.2 Discussion of the Photocurrent
-B`;Sx 6.2.1 Kinematics of Internal Photoemission in a Polycrystalline Sample
HjV^6oP 6.2.2 Primary and Secondary Cones in the Photoemission from a Real Solid
>n` OLHg; 6.2.3 Angle-Integrated and Angle-Resolved Data Collection
j-A
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*wh'4i}u 6.3.1 Band Structure Regime
tgrQ$Yjk 6.3.2 XPS Regime
-R&h?ec 6.3.3 Surface Emission
XWB>'
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/~AwX8X 6.4 Thermal Effects
\&e+f#!u 6.5 Dipole Selection Rules for Direct Optical Transitions
YjdH7.js References
`5q`ibyPI Dq-h`lh!D# 7.Band Structtire and Angular-Resolved Photoelectron Spectra
?*4]LuK6 7.1 Free-Electron Final—State Model
zIdQ^vm8Q 7.2 Methods Employing Calculated Band Structures
W^yF5 7.3 Methods for the Absolute Determination of the Crystal Momentum
- MBK/ 7.3.1 Triangulation or Energy Coincidence Method
ym${4 7.3.2 Bragg Plane Method: Variation of External Emission Angle at Fixed Photon Frequency (Disappearance/Appearance Angle Method
G~m(&,:Mu 7.3.3 Bragg Plane Method: Variation of Photon Energy at Fixed Emission Angle (Symmetry Method)
dC.uK^FuJ 7.3.4 The Surface Emission Method and Electron Damping
{J99F 7.3.5 The Very-Low-Energy Electron Diffraction Method
FWD9!M K 7.3.6 The Fermi Surface Method
9V"^F.> 7.3.7 Intensities and Their Use in Band-Structure Determinations
+<3tv&" 7.3.8 Summary
?]P&3UU>0z 7.4 Experimental Band Structures
hs/nM"V
7.4.1 One- and Two-Dimensional Systems
px-*uh< 7.4.2 Three-Dimensional Solids: Metals and Semiconductors
E6@+w. VVO 7..4.3UPS Band Structures and XPS Density of States
"`&?<82 7.5 A Comment
65<p: References
ly^F?.e- } [75`pC~O 8.Surface States, Surface Effects
;9prsvf
8.1 Theoretical Considerations
pwu5Fxn) 8.2 Experimental Results on Surface States
~xHr/: 8.3 Quantum-Well States
x"N,oDs 8.4 Surface Core-Level Shifts
x#ouR+< References
(Ojg~P4;& H M76%9! 9.Inverse Photoelectron Spectroscopy
bk>M4l61 9.1 Surface States
G1P m!CM= 9.2 Bulk Band Structures
9Y/c<gbY 9.3 Adsorbed Molecules
f'#7i@Je References
{8UBxFIM( z?yADYr9 10. Spin-Polarized Photoelectron Spectroscopy
!(o)*S 10.1 General Description
Ay2|@1e 10.2 Examples of Spin-Polarized Photoelectron Spectroscopy
!\!fd(BN 10.3 Magnetic Dichroism
IWMqmCbv References
E^|b3G6T IAtc^'l# 11. Photoelectron Diffraction
8`^I.tD 11.1 Examples
,q:6[~n 11.2 Substrate Photoelectron Diffraction
31bKgU{ 11.3 Adsorbate Photoelectron Diffraction
PHz/^p3F 11.4 Fermi Surface Scans
b%v1]a[ References
O:u^jcXA HD`Gi0 Appendix
}K&K{ 9} A.1 Table of Binding Energies
yyiZV\ / A.2 Surface and Bulk Brillouin Zones of the Three Low-Index Faces of a Face—Centered Cubic(fcc)Crystal Face
0|NbU A.3 Compilation of Work Functions
UQTt;RS*zS References
X@\! \ Index