光电子谱技术是研究原子、分子、固体和表面电子
结构的一种非常有效的手段。本书全面
系统地介绍了
光电子谱技术的
原理和应用,并简明讨论了逆光发射、自旋极化光发射和
光电子衍射等现象。本书是一本非常实用的光电子谱技术的专著,内容几乎覆盖了光电子研究的所有领域。其特点是紧密联系实验,并利用理论详细解释实验结果,达到理论和应用的有机结合。书中还收集了大量的实际
材料的光电子谱分析,同时给出了大量的实验数据,以便于读者的查阅。总之,该书既是一本很有价值的参考书,又可作为初学者的入门教材。
(7R?T} i=gZ8Q=H 作者在该领域做出了杰出的贡献。在第3版中,作者介绍了大量最新研究成果,并对光电子谱技术很多方面给出了有深刻见解的讨论。
;XN|dq >bW=oTFz 读者对象:适用于凝聚态
物理学、材料物理学和光电子学等专业的高年级本科生、研究生和相关专业的科研人员。
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XFS~ U,#~9 目录
^FLs_=E 1. Introduction and Basic Principles
2{=]Pf 1.1 Historical Development
%,T*[d&i 1.2 The Electron Mean Free Path
`s7pM 1.3 Photoelectron Spectroscopy and Inverse Photoelectron Spectroscopy
"Vp
nr +6 1.4 Experimental Aspects
vJ&_-CX 1.5 Very High Resolution
.a@12J(I 1.6 The Theory of Photoemission
#gC[L=01 1.6.1 Core-Level Photoemission
J
p?XV<3Z 1.6.2 Valence-State Photoemission
!6(3Y 1.6.3 Three-Step and One-Step Considerations
hY&Yp^"}]^ 1.7 Deviations from the Simple Theory of Photoemission
gC1LQ!:;Oi References
z.8/[) ~q ^o|? 2. Core Levels and Final States
\;&;K'
2.1 Core-Level Binding Energies in Atoms and Molecules
=|?`5!A 2.1.1 The Equivalent-Core Approximation
;E.]:Ia~ 2.1.2 Chemical Shifts
_LaG%* R6 2.2 Core-Level Binding Energies in Solids
%/A>'p,~ 2.2.1 The Born-Haber Cycle in Insulators
c>LP}PGk 2.2.2 Theory of Binding Energies
EVPQe- 2.2.3 Determination of Binding Energies and Chemical Shifts from Thermodynamic Data
5MnP6(3$ 2.3 Core Polarization
UePkSz9EU 2.4 Final-State Multiplets in Rare-Earth Valence Bands
Jpapl%7v 2.5 Vibrational Side Bands
l eC!Yj 2.6 Core Levels of Adsorbed Molecules
E
f\|3D_ 2.7 Quantitative Chemical Analysis from Core-Level Intensities
|]< 3cW+ References
x9 > ho R%jOgZG 3. Charge-Excitation Final States: Satellites
tW UI?\ 3.1 Copper Dihalides; 3d Transition Metal Compounds
s;vt2>;q+e 3.1.1 Characterization of a Satellite
NW[K/`-CTH 3.1.2 Analysis of Charge-Transfer Satellites
NVMn7H}>
3.1.3 Non-local Screening
a
8k2*u 3.2 The 6-eV Satellite in Nickel
j-K[]$ 3.2.1 Resonance Photoemission
:BPgDLL, 3.2.2 Satellites in Other Metals
D>5)',D8xi 3.3 The Gunnarsson-Sch6nhammer Theory
Ph=NH8 3.4 Photoemission Signals and Narrow Bands in Metals
^{}G4BEY References
.)tv'V/ RhowhQ) G 4. Continuous Satellites and Plasmon Satellites: XPS Photoemission in Nearly Free Electron Systems
:M"+ 4.1 Theory
8$}<4 `39 4.1.1 General
g7zl5^o3j 4.1.2 Core-Line Shape
6BV 6<PHJ 4.1.3 Intrinsic Plasmons
@7nZjrH 4.1.4 Fxtrinsic FAectron Scattering: Plasmons and Background
:`N&BV 4.1.5 The Total Photoelectron Spectrum
0Q{lyu 4.2 Experimental Results
j#//U2VdN 4.2.1 The Core Line Without Plasmons
xrg"/?84 4.2.2 Core-Level Spectra Including Plasmoas
D)-LZbPa 4.2.3 Valence-Band Spectra of the Simple Metals
@6"MhF 4.2.4 Simple Metals: A General Comment
tNY;wl:wp 4.3 The Background Correction
d~<$J9% References
|Y!^E %* J@-'IJ 5. Valence Orbitals in Simple Molecules and Insulating Solids
{bXN[=j 5.1 UPS Spectra of Monatomic Gases
l!,tssQ 5.2 Photoelectron Spectra of Diatomic Molecules
M+&~sX*a 5.3 Binding Energy of the H2 Molecule
a[K&;) 5.4 Hydrides Isoelectronic with Noble Gases
ql@2<V{ Neon (Ne)
LLgw1 @-D Hydrogen Fluoride (HF)
g4^-B Water (H2O)
V48_aL Ammonia (NH3)
c[-N A Methane (CH4)
|.c4y* 5.5 Spectra of the Alkali HMides
8xlj,}QO\ 5.6 Transition Metal Dihalides
OL\-SQ& 5.7 Hydrocarbons
A$wC!P|; 5.7.1 Guidelines for the Interpretation of Spectra from Free Molecules
AW r2Bv 5.7.2 Linear Polymers
#2^0z`-\_z 5.8 Insulating Solids with Valence d Electrons
\aJ>? 5.8.1 The NiO Problem
.!4'Y} 5.8.2 Mort Insulation
2Z{?3mAb; 5.8.3 The Metal-Insulator Transition;the Ratio of the Correlation Energy and the Bandwidth;Doping
`<tRfl}qs 5.8.4Band Structures of Transition Metal Compounds
h{)m}"n<R 5.9 High—Temperature Superconductors
XNa{_3v 5.9.1valence-Band Electronic Structure;Polycrystalline Samples
U
'{PpZ 5.9.2 Dispersion Relations in High Temperature Superconductors;Single Crystals
oZ2:% 5.9.3 The Superconducting Gap
Kl. *Q 5.9.4 Symmetry of the Order Parameter in the High-Temperature SuDerconductors
w,IJ44f ^% 5.9.5 Core—Level Shifts
x_7$g<n 5.10 The Fermi Liquid and the Luttinger Liquid
;}Jv4Z 5.11 Adsorbed Molecules
.f$2-5q 5.11.1 Outline
C
O6}D 5.11.2 CO on Metal Surfaces
cpk\;1&t References
]2-Qj)mZ] sNx_9pJs4 6.Photoemission of Valence Electrons froill Metallic Solids in the OHe-Electron Approximation
&W>\Vl1 6.1 Theory of Photoemission:A Summary of the Three-Step Model
HW[&q 6.2 Discussion of the Photocurrent
K["rr/ 6.2.1 Kinematics of Internal Photoemission in a Polycrystalline Sample
BQfnoF 6.2.2 Primary and Secondary Cones in the Photoemission from a Real Solid
;jgf,fbM 6.2.3 Angle-Integrated and Angle-Resolved Data Collection
wp~}1]g 6.3 Photoemission from the Semi—infinite Crystal:The Inverse LEED Formalism
?Q_ @@) 6.3.1 Band Structure Regime
yM 7{v$X0 6.3.2 XPS Regime
ll5;09 6.3.3 Surface Emission
B}04E^ 6.3.4 One-Step Calculations
Cj#wY 6.4 Thermal Effects
]n4PM=hz 6.5 Dipole Selection Rules for Direct Optical Transitions
x6K_!L*Fx] References
+\+j/sa !Mw/j`* 7.Band Structtire and Angular-Resolved Photoelectron Spectra
6KGT?d 7.1 Free-Electron Final—State Model
D<v<
: 7.2 Methods Employing Calculated Band Structures
ir'<H<t2 7.3 Methods for the Absolute Determination of the Crystal Momentum
ox SSEs 7.3.1 Triangulation or Energy Coincidence Method
;*rGZ?%* 7.3.2 Bragg Plane Method: Variation of External Emission Angle at Fixed Photon Frequency (Disappearance/Appearance Angle Method
7s%D(;W_Mo 7.3.3 Bragg Plane Method: Variation of Photon Energy at Fixed Emission Angle (Symmetry Method)
P:g!~&Q 7.3.4 The Surface Emission Method and Electron Damping
;jxX /c 7.3.5 The Very-Low-Energy Electron Diffraction Method
~0CNCP 7.3.6 The Fermi Surface Method
t!wbT79/ 7.3.7 Intensities and Their Use in Band-Structure Determinations
4(,.<# 7.3.8 Summary
5!ngM 7.4 Experimental Band Structures
"6]oi*_8 7.4.1 One- and Two-Dimensional Systems
~d&&\EZ 7.4.2 Three-Dimensional Solids: Metals and Semiconductors
kQU4s)J 7..4.3UPS Band Structures and XPS Density of States
"`K_5"F 7.5 A Comment
O4`.ohAZ References
X,3"4 SK ]|F`;} 7 8.Surface States, Surface Effects
.;31G0<w2 8.1 Theoretical Considerations
~98q1HgS]D 8.2 Experimental Results on Surface States
z~ Zm1tZs 8.3 Quantum-Well States
e }O&_j- 8.4 Surface Core-Level Shifts
YQ+8lANC References
HpbwW=;V W+u@UJi 9.Inverse Photoelectron Spectroscopy
bBINjs8C_ 9.1 Surface States
o?O ZsA 9.2 Bulk Band Structures
u9:sj 9.3 Adsorbed Molecules
2KXFXR References
4grV2xtX yq, qS0Fo 10. Spin-Polarized Photoelectron Spectroscopy
]l }v 10.1 General Description
L]=mQo 10.2 Examples of Spin-Polarized Photoelectron Spectroscopy
?p6@uM\Q7 10.3 Magnetic Dichroism
bHq.3; References
Qv,ORm
h5 1V5N)ty 11. Photoelectron Diffraction
^Zpz@T>m 11.1 Examples
jB -Ad8 11.2 Substrate Photoelectron Diffraction
%Lx#7bR U 11.3 Adsorbate Photoelectron Diffraction
GQ
Flt_ 11.4 Fermi Surface Scans
e]1)_;b* References
!]"M]tyv\ UptKN|S&V Appendix
lx$Z/f A.1 Table of Binding Energies
aIT0t0. A.2 Surface and Bulk Brillouin Zones of the Three Low-Index Faces of a Face—Centered Cubic(fcc)Crystal Face
s'/_0 A.3 Compilation of Work Functions
CZy!nR! References
M+-odLltw Index